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A D Bianchi

Publications and source records attributed to A D Bianchi.

5 recordsLinked to original sources

Magneto-optical evidence of double exchange in a percolating lattice.

Substituting Eu by Ca in ferromagnetic EuB6 leads to a percolation limited magnetic ordering. We present and discuss magneto-optical data of the Eu(1-x)Ca(x)B6 series, based on measurements of the reflectivity R(omega) from the far infrared up to the ultraviolet, as a function of temperature and magnetic field. Via the Kramers-Kronig transformation of R(omega) we extract the complete absorption spectra of samples with different values of x. The change of the spectral weight in the Drude component by increasing the magnetic field agrees with a scenario based on the double-exchange model, and suggests a crossover from a ferromagnetic metal to a ferromagnetic Anderson insulator upon increasing Ca content at low temperatures.

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Percolation and the colossal magnetoresistance of Eu-based hexaboride.

Upon substituting Ca for Eu in the local-moment ferromagnet EuB6, the Curie temperature T(C) decreases substantially with increasing dilution of the magnetic sublattice and is completely suppressed for x<or=0.3. The Ca substitution leads to significant changes of the electronic properties across the EuxCa1-xB6 series. Electron microscopy data for x approximately 0.27 indicate a phase separation into Eu- and Ca-rich clusters of 5 to 10 nm diameter, leading to percolation-type phenomena in the electrical transport properties. The related critical concentration x(p) is approximately 0.3. For x approximately 0.27, we observe colossal negative magnetoresistance effects at low temperatures, similar in magnitude as those reported for manganese oxides.

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Optical evidence for a spin-filter effect in the charge transport of Eu0.6Ca0.4B6.

We have measured the optical reflectivity R(omega) of Eu0.6Ca0.4B6 as a function of temperature (T) between 1.5 and 300 K and in external magnetic fields (H) up to 7 T. R(omega) increases with decreasing T and increasing H field, but the plasma edge feature does not exhibit the sharp onset and steep slope that is observed in EuB6. The analysis of the H-field dependence of the low-T optical conductivity confirms the previously observed exponential decrease of the electrical resistivity upon increasing bulk magnetization at constant T. The individual exponential magnetization dependences of the plasma frequency and scattering rate are also extracted from the optical data.

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First-order transition from a Kondo insulator to a ferromagnetic metal in single crystalline FeSi(1-x)Ge(x).

The phase diagram of FeSi(1-x)Ge(x), obtained from magnetic, thermal, and transport measurements on single crystals, shows a discontinuous transition from Kondo insulator to ferromagnetic metal with x at a critical concentration, x(c) approximately 0.25. The gap of the insulating phase strongly decreases with x. The specific heat gamma coefficient appears to track the density of states of a Kondo insulator. The phase diagram is consistent with an insulator-metal transition induced by a reduction of the hybridization with x in conjunction with disorder on the Si/Ge ligand site.

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Bulk band gaps in divalent hexaborides.

Complementary angle-resolved photoemission and bulk-sensitive k-resolved resonant inelastic x-ray scattering of divalent hexaborides reveal a >1 eV X-point gap between the valence and conduction bands, in contradiction to the band overlap assumed in several models of their novel ferromagnetism. This semiconducting gap implies that carriers detected in transport measurements arise from defects, and the measured location of the bulk Fermi level at the bottom of the conduction band implicates boron vacancies as the origin of the excess electrons. The measured band structure and X-point gap in CaB6 additionally provide a stringent test case for many-body quasiparticle band calculations.

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