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A Georges

Publications and source records attributed to A Georges.

At least 19 recordsLinked to original sources

Breakup of the Fermi surface near the mott transition in low-dimensional systems.

We investigate the Mott transition in weakly coupled one-dimensional (1D) fermionic chains. Using a generalization of dynamical mean field theory, we show that the Mott gap is suppressed at some critical hopping t{ perpendicular}{c2}. The transition from the 1D insulator to a 2D metal proceeds through an intermediate phase where the Fermi surface is broken into electron and hole pockets. The quasiparticle spectral weight is strongly anisotropic along the Fermi surface, both in the intermediate and metallic phases. We argue that such pockets would look like "arcs" in photoemission experiments.

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Coherent peaks and minimal probing depth in photoemission spectroscopy of Mott-Hubbard systems.

We have measured hard x-ray photoemission spectra of pure vanadium sesquioxide (V(2)O(3)) across its metal-insulator transition. We show that, in the metallic phase, a clear correlation exists between the shakedown satellites observed in the vanadium 2p and 3p core-level spectra and the coherent peak measured at the Fermi level. Comparing experimental results and dynamical mean-field theory calculations, we estimate the Hubbard energy U in V(2)O(3) (4.20+/-0.05 eV). From our bulk-sensitive photoemission spectra we infer the existence of a critical probing depth for investigating electronic properties in strongly correlated solids.

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Time evolution of the electronic structure of 1T-TaS2 through the insulator-metal transition.

Femtosecond time-resolved photoemission is used to investigate the time evolution of electronic structure in the Mott insulator 1T-TaS2. A collapse of the electronic gap is observed within 100 femtoseconds after optical excitation. The photoemission spectra and the spectral function calculated by dynamical mean field theory show that this insulator-metal transition is driven solely by hot electrons. A coherently excited lattice displacement results in a periodic shift of the spectra lasting for 20 ps without perturbing the insulating phase. This capability to disentangle electronic and phononic excitations opens new directions to study electron correlation in solids.

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The alpha-gamma transition of cerium is entropy driven.

We emphasize, on the basis of experimental data and theoretical calculations, that the entropic stabilization of the gamma phase is the main driving force of the alpha-gamma transition of cerium in a wide temperature range below the critical point. Using a formulation of the total energy as a functional of the local density and of the f-orbital local Green's functions, we perform dynamical mean-field theory calculations within a new implementation based on the multiple linear muffin tin orbital (LMTO) method, which allows us to include semicore states. Our results are consistent with the experimental energy differences and with the qualitative picture of an entropy-driven transition, while also confirming the appearance of a stabilization energy of the alpha phase as the quasiparticle Kondo resonance develops.

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Non-Fermi-liquid behavior and double-exchange physics in orbital-selective Mott systems.

We study a multiband Hubbard model in its orbital-selective Mott phase, in which localized electrons in a narrow band coexist with itinerant electrons in a wide band. The low-energy physics of this phase is shown to be given by a generalized double-exchange model. The high-temperature disordered phase thus differs from a Fermi liquid, and displays a finite scattering rate of the conduction electrons at the Fermi level, which depends continuously on the spin anisotropy.

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Mott transition and Kondo screening in f-electron metals.

We study how a finite hybridization between a narrow correlated band and a wide conduction band affects the Mott transition. At zero temperature, the hybridization is found to be a relevant perturbation, so that the Mott transition is suppressed by Kondo screening. In contrast, a first-order transition remains at finite temperature, separating a local-moment phase and a Kondo-screened phase. The first-order transition line terminates in two critical end points. Implications for experiments on f-electron materials such as the cerium alloy Ce0.8La0.1Th0.1 are discussed.

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Interaction-induced adiabatic cooling and antiferromagnetism of cold fermions in optical lattices.

We propose an interaction-induced cooling mechanism for two-component cold fermions in an optical lattice. It is based on an increase of the spin entropy upon localization, an analogue of the Pomeranchuk effect in liquid helium 3. We discuss its application to the experimental realization of the antiferromagnetic phase. We illustrate our arguments with dynamical mean-field theory calculations.

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Sound velocity anomaly at the mott transition: application to organic conductors and V2O3.

Close to the Mott transition, lattice degrees of freedom react to the softening of electron degrees of freedom. This results in a change of lattice spacing, a diverging compressibility, and a critical anomaly of the sound velocity. These effects are investigated within a simple model, in the framework of dynamical mean-field theory. The results compare favorably to recent experiments on the layered organic-conductor kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl. We predict that effects of a similar magnitude are expected for V(2)O(3), despite the much larger value of the elastic modulus of this material.

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Dynamical singlets and correlation-assisted Peierls transition in VO2.

A theory of the metal-insulator transition in vanadium dioxide from the high- temperature rutile to the low- temperature monoclinic phase is proposed on the basis of cluster dynamical mean-field theory, in conjunction with the density functional scheme. The interplay of strong electronic Coulomb interactions and structural distortions, in particular, the dimerization of vanadium atoms in the low-temperature phase, plays a crucial role. We find that VO2 is not a conventional Mott insulator, but that the formation of dynamical V-V singlet pairs due to strong Coulomb correlations is necessary to trigger the opening of a Peierls gap.

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Mott transition and suppression of orbital fluctuations in orthorhombic 3d1 perovskites.

Using t(2g) Wannier functions, a low-energy Hamiltonian is derived for orthorhombic 3d(1) transition-metal oxides. Electronic correlations are treated with a new implementation of dynamical mean-field theory for noncubic systems. Good agreement with photoemission data is obtained. The interplay of correlation effects and cation covalency (GdFeO3-type distortions) is found to suppress orbital fluctuations in LaTiO3 and even more in YTiO3, and to favor the transition to the insulating state.

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Changes in type B natriuretic peptide (BNP) concentrations during cardiac valve replacement.

OBJECTIVE: The aim of our study was to investigate the ability of BNP levels to reveal the immediate post-surgery cardiac function improvement. We measured the perioperative variations in BNP concentrations in patients scheduled for cardiac surgery with cardiopulmonary bypass (CPB), chronic mitral regurgitation, valvular aortic stenosis, or myocardial ischaemia. METHODS: Three groups were included: patients with coronary artery bypass graft (CABG, group I, n = 14), aortic (AVR, group II, n = 14) or mitral (MVR, group III, n = 7) valve replacement. BNP assay was performed at the induction of anesthesia, immediately after the CPB, at the arrival in the intensive care unit, 4 h, 8 h and 12 h after the arrival in ICU. RESULTS AND CONCLUSION: The occurring variation in BNP levels after the operation is an increase whatever the corrective surgery, underlying the relative lack of specificity of BNP with regard to the cardiac pathology. Besides iatrogenic cardioplegia one can supposes that cardiac surgery involves other major stimuli such as anesthesia, sternotomia, hemodynamics, post-operative that could influence in a non specific way BNP levels.

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Universality and critical behavior at the Mott transition.

We report conductivity measurements of Cr-doped V2O3 using a variable pressure technique. The critical behavior of the conductivity near the Mott insulator to metal critical endpoint is investigated in detail as a function of pressure and temperature. The critical exponents are determined, as well as the scaling function associated with the equation of state. The universal properties of a liquid-gas transition are found. This is potentially a generic description of the Mott critical endpoint in correlated electron materials.

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Mott transition and transport crossovers in the organic compound kappa-(BEDT-TTF)2Cu[N(CN)2]Cl.

We have performed in-plane transport measurements on the two-dimensional organic salt kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl. A variable (gas) pressure technique allows for a detailed study of the changes in conductivity through the insulator-to-metal transition. We identify four different transport regimes as a function of pressure and temperature (corresponding to insulating, semiconducting, "bad metal," and strongly correlated Fermi-liquid behaviors). Marked hysteresis is found in the transition region, which displays complex physics that we attribute to strong spatial inhomogeneities. Away from the critical region, good agreement is found with a dynamical mean-field calculation of transport properties using the numerical renormalization group technique.

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Spectroscopic signatures of a bandwidth-controlled Mott transition at the surface of 1T-TaSe2.

High-resolution angle-resolved photoemission data show that a metal-insulator Mott transition occurs at the surface of the quasi-two-dimensional compound 1T-TaSe2. The transition is driven by the narrowing of the Ta 5d band induced by a temperature-dependent modulation of the atomic positions. A dynamical mean-field theory calculation of the spectral function of the half-filled Hubbard model captures the main qualitative feature of the data, namely, the rapid transfer of spectral weight from the observed quasiparticle peak at the Fermi surface to the Hubbard bands, as the correlation gap opens up.

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First-principles approach to the electronic structure of strongly correlated systems: combining the GW approximation and dynamical mean-field theory.

We propose a dynamical mean-field approach for calculating the electronic structure of strongly correlated materials from first principles. The scheme combines the GW method with dynamical mean-field theory, which enables one to treat strong interaction effects. It avoids the conceptual problems inherent to conventional "LDA+DMFT," such as Hubbard interaction parameters and double-counting terms. We apply a simplified version of the approach to the electronic structure of nickel and find encouraging results.

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Deconfinement transition and Luttinger to Fermi liquid crossover in quasi-one-dimensional systems.

We investigate a system of one-dimensional Hubbard chains of interacting fermions coupled by interchain hopping. Using a generalization of the dynamical mean-field theory we study the deconfinement transition from a Mott insulator to a metal and the crossover between Luttinger and Fermi liquid phases. One-particle properties, local spin response, and interchain optical conductivity are calculated. Possible applications to organic conductors are discussed.

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Dynamical mean-field theory of resonating-valence-bond antiferromagnets.

We propose a theory of the spin dynamics of frustrated quantum antiferromagnets, which is based on an effective action for a plaquette embedded in a self-consistent bath. This approach, supplemented by a low-energy projection, is applied to the Kagomé antiferromagnet. We find that a spin-liquid regime extends to very low energy, in which local correlation functions have a slow decay in time, well described by power-law behavior and omega/T scaling of the response function: chi(") (omega) is proportional to omega(-alpha)F (omega/T).

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Assessment of brain natriuretic peptide in patients with suspected heart failure: comparison with radionuclide ventriculography data.

BACKGROUND: The aim of the study was to prospectively evaluate patients with suspected or known heart disease using plasma brain natriuretic peptide (BNP) measurement and radionuclide ventriculography to examine whether left ventricular dysfunction is associated with an abnormal rise of BNP concentration. METHODS: Patients (n=153) and controls (n=14) underwent radionuclide ventriculography to determine Left ventricular Ejection Fraction (LVEF) and measurement of plasma BNP concentration using a commercial kit. RESULTS: Plasma BNP concentration in controls was significantly lower than that in patients whatever the stage of the disease, significantly lower than that of patients with normal LVEF (LVEF>55%); than that of patients with altered LVEF (LVEF< or =40%); and than that of patients with moderately reduced LVEF (40%<LVEF< or =5%). Comparisons between groups of patients showed that the more severe the disease, the higher the BNP level. From the ROC curve, a plasma BNP concentration of 52 pg/ml was attached to a 85% sensitivity and 82% specificity in identifying patients with LVEF< or =40%. CONCLUSIONS: Plasma BNP concentration provides a reliable and sensitive marker of LV systolic dysfunction evaluated by a nuclear medicine technique, and could be a potential screening test to identify patients for additional investigations.

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