Biomedical subjects
Publications and source records attributed to A Mysyrowicz.
By studying the conical emission of a blue femtosecond laser filament in air, it is shown that self-improvement of the beams' spatial mode quality occurs for a self-guided laser pulse.
Femtosecond laser filamentation is studied in a broadband amplifying medium, sapphire doped with electronically excited Ti ions. Evidence for fluence amplification of self-guided pulses, increase of filamentation length, as well as a lowering of the input laser power necessary for filamentation is reported.
We calculate pulse self-compression of a 30 fs laser pulse traversing gas with different pressure gradients. We show that an appropriate density profile brings significant improvement to the self-compression by filamentation. Under an optimal pressure gradient, the pulse duration is reduced to the single optical cycle limit over a long distance, allowing easy extraction into an interaction chamber.
Using time-resolved 1s-2p excitonic Lyman spectroscopy, we study the orthoexciton-to-paraexciton transfer, following the creation of a high density population of ultracold 1s orthoexcitons by resonant two-photon excitation with femtosecond pulses. An observed fast exciton-density dependent conversion rate is attributed to spin exchange between pairs of orthoexcitons. Implication of these results on the feasibility of Bose-Einstein condensation of paraexcitons in Cu(2)O is discussed.
We show that it is possible to organize regular filamentation patterns in air by imposing either strong field gradients or phase distortions in the input-beam profile of an intense femtosecond laser pulse. A comparison between experiments and 3+1 dimensional numerical simulations confirms this concept and shows for the first time that a control of the transport of high intensities over long distances may be achieved by forcing this well ordered propagation regime. In this case, deterministic effects prevail in multiple femtosecond filamentation, and no transition to the optical turbulence regime is obtained [Phys. Rev. Lett. 83, 2938 (1999)]].
Radiation is almost completely reflected within the exciton-polariton stop band of a semiconductor, as in the typical case of CuCl. We predict, however, that a coherently driven exciton-biexciton transition allows for the propagation of a probe light beam within the stop band. The phenomenon is reminiscent of electromagnetically induced transparency effects occurring in three-level atomic systems, except that it here involves delocalized electronic excitations in a crystalline structure via a frequency and wave-vector selective polaritonic mechanism. A well-developed transparency, favored by the narrow linewidth of the biexciton, is established within the stop band where a probe pulse may propagate with significant delays. The transparency window can be controlled via the pump beam detuning and intensity.
Most long-path remote spectroscopic studies of the atmosphere rely on ambient light or narrow-band lasers. High-power femtosecond laser pulses have been found to propagate in the atmosphere as dynamically self-guided filaments that emit in a continuum from the ultraviolet to the infrared. This white light exhibits a directional behavior with enhanced backward scattering and was detected from an altitude of more than 20 kilometers. This light source opens the way to white-light and nonlinear light detection and ranging applications for atmospheric trace-gas remote sensing or remote identification of aerosols. Air ionization inside the filaments also opens promising perspectives for laser-induced condensation and lightning control. The mobile femtosecond-terawatt laser system, Teramobile, has been constructed to study these applications.
We present experimental results from the collision of weak ultrashort pulses with relativistic ionization fronts in copropagation and counterpropagation. The observed frequency upshifts of the probe pulses provide not only information about the electron density of the ionization front but also reveal the fine structure of the front. The connection between the correlation lengths for copropagation and counterpropagation and the longitudinal and transverse dimensions of the ionization front is also demonstrated thus showing the feasibility of using the frequency upshift experienced by short probe pulses to fully characterize relativistic ionization fronts and other relativistic coherent structures in laser-produced plasmas.
A reversible coupling between photon pair states and a long-lived, highly coherent biexciton wave in CuCl allows efficient phase-sensitive two-photon amplification or attenuation of ultrashort light pulses. We demonstrate a gain of 350 cm(-1) for a pump intensity of 1 MW/cm(2), nearly 2 orders of magnitude higher than that achievable with conventional parametric crystal amplifiers. We develop a theoretical model that describes this new type of parametric converter where the light pump is replaced by a coherent biexciton wave and show that it is well suited for the generation of entangled photons and the squeezing of an optical beam with ultrafast time gating.
Bulk damage induced by fs IR laser pulses in silica is investigated both experimentally and numerically. In a strong focusing geometry, a first damage zone is followed by a narrow track with submicron width, indicating a filamentary propagation. The shape and size of the damage tracks are shown to correspond to the zone where the electron density created by optical field ionization and avalanche is close to 10(20) cm(-3). The relative role of avalanche and photoionization is studied. The plasma density produced in the wake of the pulse is shown to saturate around 2-4x10(20) cm(-3).
We report self-guided propagation of ultrashort IR laser pulses in fused silica over several Rayleigh lengths. Self-guiding is accompanied by pulse splitting and time compression. Numerical simulations involving pulse self-focusing, temporal dispersion, and multiphoton ionization are found to be in good agreement with the experimental results. They show that a quasidynamic equilibrium between multiphoton ionization and self-focusing drives the filamentation process, while temporal dispersion plays a negligible role.
The filament due to the self-guided propagation of an infrared femtosecond laser pulse in atmospheric-pressure air is used to trigger and guide an electric discharge. The long low density plasma channel due to the filament is first heated by the Joule effect during an initial transient plasma stage. The heated channel of recombined gas then hydrodynamically expands radially. The onset of a discharge starts when the density depression on axis reaches the threshold discharge value. This model is supported by detailed experimental and numerical analysis.
We report experiments showing the breakup and the merging of filaments formed by the modulational instability of femtosecond optical pulses in air. For input powers as high as 25 times the self-focusing threshold, the beams are shown to split into two spots, which coalesce into a self-guided beam. This effect occurs in an optically Kerr regime and plays an important role in the guiding process. Numerical simulations and theoretical estimates both support the comparison with the experimental data.
We report a drastic reduction of air resistivity following the passage of a self-guided femtosecond pulse from a Ti:sapphire laser system at 800 nm with energies per pulse between 1 and 14 mJ and a pulse duration of 120 fs. Connected plasma filaments with a length that can exceed 150 cm are created by these pulses. The presence of a conducting plasma channel results from multiphoton ionization of air molecules in the filament core.
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