Biomedical subjects

D A Jaroszynski

Publications and source records attributed to D A Jaroszynski.

8 recordsLinked to original sources

PubMed2006

Temporally resolved electro-optic effect.

The electro-optic effect between an ultrafast optical probe pulse and an ultrashort terahertz pulse is shown to depend on the time derivatives of the product of the probe and terahertz electric fields. Application of this theory to temporally resolved single-shot terahertz detection techniques, where the electro-optic effect is temporally localized within an optical probe pulse, shows that the description presented here differs fundamentally and verifiably from that commonly used in literature.

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PubMed2006

Radiation sources based on laser-plasma interactions.

Plasma waves excited by intense laser beams can be harnessed to produce femtosecond duration bunches of electrons with relativistic energies. The very large electrostatic forces of plasma density wakes trailing behind an intense laser pulse provide field potentials capable of accelerating charged particles to high energies over very short distances, as high as 1GeV in a few millimetres. The short length scale of plasma waves provides a means of developing very compact high-energy accelerators, which could form the basis of compact next-generation light sources with unique properties. Tuneable X-ray radiation and particle pulses with durations of the order of or less than 5fs should be possible and would be useful for probing matter on unprecedented time and spatial scales. If developed to fruition this revolutionary technology could reduce the size and cost of light sources by three orders of magnitude and, therefore, provide powerful new tools to a large scientific community. We will discuss how a laser-driven plasma wakefield accelerator can be used to produce radiation with unique characteristics over a very large spectral range.

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PubMed2005

Superradiant linear Raman amplification in plasma using a chirped pump pulse.

A theoretical and numerical investigation of small-signal Raman backscattering from a chirped pump pulse in plasma shows that an ultrashort probe pulse will grow superradiantly, i.e., with an amplitude that scales with the propagation length while contracting self-similarly. These features are commonly associated with the nonlinear stages of Raman amplification in the pump depletion and Compton regimes. We show that the superradiant scaling results in very broad-bandwidth amplification due to gain distributed in frequency as well as spatially. Since different frequencies excite the plasma at different positions, wave breaking is avoided, and prepulses and pedestals are substantially suppressed. Linear chirped pulse amplification in plasma could provide a very broad-bandwidth alternative to solid state laser amplifiers, potentially usable for optical pulses a few cycles in duration.

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PubMed2005

Efficiency and energy spread in laser-wakefield acceleration.

The theoretical limits on efficiency and energy spread of the laser-wakefield accelerator are investigated using a one-dimensional model. Modifications, both of the wakefield due to the electron bunch, and of the laser pulse shape due to the varying permittivity of the plasma, are described self-consistently. It is found that a short laser pulse gives a higher efficiency than a long laser pulse with the same initial energy. Energy spread can be minimized by optimizing bunch length and bunch charge such that the variation of the accelerating force along the length of the bunch is minimized. An inherent trade-off between energy spread and efficiency exists.

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PubMed2005

Interaction mechanism of some alkyl iodides with femtosecond laser pulses.

The interaction of 1-iodopropane, 2-iodopropane, 1-iodobutane, 2-iodobutane, and 1-iodopentane with (5 x 10(13-)5 x 10(15) W/cm2) femtosecond laser fields is studied by means of a time-of-flight mass spectrometer. It is found that multiphoton ionization (MPI) and field ionization (FI) processes are involved in the molecular ionization. The contribution of these processes can be distinguished using the peak profile of the ions in the mass spectra. Thus, from the mass spectra of 2-iodoropane and 2-iodobutane, it is concluded that MPI processes are taking place even for Keldysh parameter values gamma approximately 0.3. The field ionization process depends on the characteristics of the molecular binding potential well and leads to an asymmetric charge distribution of the transient multiply charged parent ions. In the case of 1-iodobutane, the MPI processes lead to a stable doubly charged parent ion production with a laser intensity threshold higher than that found for I2+ ions. In addition, the isomers studied exhibit distinct differences in their mass spectra and their origin is discussed in detail.

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PubMed2004

Monoenergetic beams of relativistic electrons from intense laser-plasma interactions.

High-power lasers that fit into a university-scale laboratory can now reach focused intensities of more than 10(19) W cm(-2) at high repetition rates. Such lasers are capable of producing beams of energetic electrons, protons and gamma-rays. Relativistic electrons are generated through the breaking of large-amplitude relativistic plasma waves created in the wake of the laser pulse as it propagates through a plasma, or through a direct interaction between the laser field and the electrons in the plasma. However, the electron beams produced from previous laser-plasma experiments have a large energy spread, limiting their use for potential applications. Here we report high-resolution energy measurements of the electron beams produced from intense laser-plasma interactions, showing that--under particular plasma conditions--it is possible to generate beams of relativistic electrons with low divergence and a small energy spread (less than three per cent). The monoenergetic features were observed in the electron energy spectrum for plasma densities just above a threshold required for breaking of the plasma wave. These features were observed consistently in the electron spectrum, although the energy of the beam was observed to vary from shot to shot. If the issue of energy reproducibility can be addressed, it should be possible to generate ultrashort monoenergetic electron bunches of tunable energy, holding great promise for the future development of 'table-top' particle accelerators.

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PubMed2003

High-temporal-resolution, single-shot characterization of terahertz pulses.

A technique for noncollinear cross correlation of electro-optic modulated optical pulses is presented for the single-shot characterization of terahertz waveforms and is compared to established electro-optic terahertz characterization methods. This technique is free from the limitations on time resolution and faithful reproduction of previously demonstrated single-shot amplitude modulation spectral encoding.

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PubMed2002

Femtosecond laser time-of-flight mass spectrometry of labile molecular analytes: laser-desorbed nitro-aromatic molecules.

Femtosecond laser time-of-flight mass spectra of solid samples of trinitrobenzene (TNB), trinitrotoluene (TNT) and trinitrophenol (TNP) have been recorded. Desorption of the solid samples was enacted by the fourth harmonic output (266 nm) of a 5 ns Nd:YAG laser. Subsequent femtosecond post-ionisation of the plume of neutral molecules was achieved using 800 nm laser pulses of 80 fs duration. Mass spectra have been recorded for desorption laser intensities from 2-6 x 10(9) W cm(-2) with ionisation laser intensities between 2 x 10(14) and 6 x 10(15) W cm(-2). Femtosecond laser ionisation has been shown to be capable of generating precursor and characteristic high-mass fragment ions for labile nitro-aromatic molecules commonly used in high-explosive materials. This feature is critical in the future development of femtosecond laser-based analytical instruments that can be used for complex molecular identification and quantitative analysis of environmentally important labile molecules. Furthermore, a comparison of femtosecond post-ionisation mass spectra with standard 70 eV electron impact data has revealed similarities in the spectra and hence the fragmentation processes.

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