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D Loss

Publications and source records attributed to D Loss.

At least 19 recordsLinked to original sources

Electron and nuclear spin dynamics in antiferromagnetic molecular rings.

We study theoretically the spin dynamics of antiferromagnetic molecular rings, such as the ferric wheel Fe10. For a single nuclear or impurity spin coupled to one of the electron spins of the ring, we calculate nuclear and electronic spin correlation functions and show that nuclear magnetic resonance (NMR) and electron spin resonance (ESR) techniques can be used to detect coherent tunneling of the Néel vector in these rings. The location of the NMR/ESR resonances gives the tunnel splitting and its linewidth an upper bound on the decoherence rate of the electron spin dynamics. We illustrate the experimental feasibility of our proposal with estimates for Fe10 molecules.

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Detection of single spin decoherence in a quantum dot via charge currents.

We consider a quantum dot attached to leads in the Coulomb blockade regime that has a spin 1 / 2 ground state. We show that, by applying an ESR field to the dot spin, the stationary current in the sequential tunneling regime exhibits a new resonance peak whose linewidth is determined by the single spin decoherence time T2. The Rabi oscillations of the dot spin are shown to induce coherent current oscillations from which T2 can be deduced in the time domain. We describe a spin inverter which can be used to pump current through a double dot via spin flips generated by ESR.

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Quantum computing in molecular magnets.

Shor and Grover demonstrated that a quantum computer can outperform any classical computer in factoring numbers and in searching a database by exploiting the parallelism of quantum mechanics. Whereas Shor's algorithm requires both superposition and entanglement of a many-particle system, the superposition of single-particle quantum states is sufficient for Grover's algorithm. Recently, the latter has been successfully implemented using Rydberg atoms. Here we propose an implementation of Grover's algorithm that uses molecular magnets, which are solid-state systems with a large spin; their spin eigenstates make them natural candidates for single-particle systems. We show theoretically that molecular magnets can be used to build dense and efficient memory devices based on the Grover algorithm. In particular, one single crystal can serve as a storage unit of a dynamic random access memory device. Fast electron spin resonance pulses can be used to decode and read out stored numbers of up to 105, with access times as short as 10-10 seconds. We show that our proposal should be feasible using the molecular magnets Fe8 and Mn12.

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Quantum dot as spin filter and spin memory

We consider a quantum dot in the Coulomb blockade regime weakly coupled to current leads and show that in the presence of a magnetic field it acts as an efficient spin filter (at the single-spin level), producing a spin-polarized current. Conversely, if the leads are fully spin polarized the up or the down state of the spin on the dot results in a large sequential or a small cotunneling current, and, thus, together with ESR techniques, the setup can be operated as a single-spin memory.

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Probing entanglement and nonlocality of electrons in a double-dot via transport and noise.

Addressing the feasibility of quantum communication with electrons we consider entangled spin states of electrons in a double-dot which is weakly coupled to leads. We show that the entanglement of two electrons in the double-dot can be detected in mesoscopic transport and noise measurements. In the Coulomb blockade and cotunneling regime the singlet and triplet states lead to phase-coherent current and noise contributions of opposite signs and to Aharonov-Bohm and Berry phase oscillations. These oscillations are a genuine two-particle effect and provide a direct measure of nonlocality in entangled states. We show that the ratio of zero-frequency noise to current is equal to the electron charge.

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