Biomedical subjects

D von der Linde

Publications and source records attributed to D von der Linde.

9 recordsLinked to original sources

PubMed2005

Observation of structural anisotropy and the onset of liquidlike motion during the nonthermal melting of InSb.

The melting dynamics of laser excited InSb have been studied with femtosecond x-ray diffraction. These measurements observe the delayed onset of diffusive atomic motion, signaling the appearance of liquidlike dynamics. They also demonstrate that the root-mean-squared displacement in the [111] direction increases faster than in the [110] direction after the first 500 fs. This structural anisotropy indicates that the initially generated fluid differs significantly from the equilibrium liquid.

Journal Article↗

PubMed2005

Atomic-scale visualization of inertial dynamics.

The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

Journal Article↗

PubMed2004

Phase-matching solutions for high-order harmonic generation in hollow-core photonic-crystal fibers.

Hollow-core photonic-crystal fibers are shown to allow phase-matched high-order harmonic generation by an isolated guided mode of pump radiation. Regimes of phase matching are analyzed for the fundamental guided mode of pump field with a wavelength around 800 nm, generating harmonics within the wavelength range of 25-50 nm in hollow photonic-crystal fibers filled with argon, krypton, and helium. Geometric parameters of the fiber structure and the pressure of the gas filling the fiber core are shown to serve as important, often orthogonal, control knobs, allowing a fine adjustment of the phase matching for high-order harmonic generation.

Journal Article↗

PubMed2004

Self-channeling of subgigawatt femtosecond laser pulses in a ground-state waveguide induced in the hollow core of a photonic crystal fiber.

Femtosecond laser pulses with powers below the blowup threshold for self-focused beams are shown to experience spatial self-action in hollow-core photonic crystal fibers filled with argon, nitrogen, and atmospheric air. Regardless of the transverse field distribution at the input of the fiber, the output beam pattern in this regime tends to a circularly symmetric profile, corresponding to a ground-state waveguide induced by laser pulses inside a hollow fiber.

Journal Article↗

PubMed2004

Generation of femtosecond anti-stokes pulses through phase-matched parametric four-wave mixing in a photonic crystal fiber.

Phase-matched parametric four-wave mixing in higher-order guided modes of a photonic crystal fiber is shown to result in an efficient decay of 40-fs 800-nm Ti:sapphire laser pump pulses into an anti-Stokes signal with a central wavelength around 590-600 nm and a Stokes signal centered at 1.25 microm. The photonic crystal fiber is designed in such a way as to minimize the group-velocity dispersion at the pump wavelength, phase match the parametric four-wave-mixing process, and reduce the group delay between the pump and the anti-Stokes pulses. The duration of the anti-Stokes pulse under these conditions, as shown by cross-correlation frequency-resolved optical gating measurements, is less than 200 fs.

Journal Article↗

PubMed2003

3/2 harmonic generation by femtosecond laser pulses in steep-gradient plasmas.

The onset of an electron parametric instability and 3/2 harmonic generation in variable-scale-length plasmas on solid surfaces using femtosecond pulses is observed. With the intensity approaching 10(18) W/cm(2), the instability threshold is already reached at plasma scale lengths of the order of the laser wavelength. A well-collimated harmonic emission with unusually broad spectrum is obtained.

Journal Article↗

PubMed2001

Femtosecond x-ray measurement of ultrafast melting and large acoustic transients.

Time-resolved x-ray diffraction with ultrashort ( approximately 300 fs), multi-keV x-ray pulses has been used to study the femtosecond laser-induced solid-to-liquid phase transition in a thin crystalline layer of germanium. Nonthermal melting is observed to take place within 300-500 fs. Following ultrafast melting we observe strong acoustic perturbations evolving on a picosecond time scale.

Journal Article↗

PubMed2000

Anharmonic lattice dynamics in germanium measured with ultrafast x-ray diffraction.

Damping of impulsively generated coherent acoustic oscillations in a femtosecond laser-heated thin germanium film is measured as a function of fluence by means of ultrafast x-ray diffraction. By simultaneously measuring picosecond strain dynamics in the film and in the unexcited silicon substrate, we separate anharmonic damping from acoustic transmission through the buried interface. The measured damping rate and its dependence on the calculated temperature of the thermal bath is consistent with estimated four-body, elastic dephasing times (T2) for 7-GHz longitudinal acoustic phonons in germanium.

Journal Article↗

PubMed1999

Detection of nonthermal melting by ultrafast X-ray diffraction.

Using ultrafast, time-resolved, 1.54 angstrom x-ray diffraction, thermal and ultrafast nonthermal melting of germanium, involving passage through nonequilibrium extreme states of matter, was observed. Such ultrafast, optical-pump, x-ray diffraction probe measurements provide a way to study many other transient processes in physics, chemistry, and biology, including direct observation of the atomic motion by which many solid-state processes and chemical and biochemical reactions take place.

Biochemistry↗