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Elbio Dagotto

Publications and source records attributed to Elbio Dagotto.

8 recordsLinked to original sources

Ferroelectricity in the magnetic E-phase of orthorhombic perovskites.

We show that the symmetry of the spin zigzag chain E phase of the orthorhombic perovskite manganites and nickelates allows for the existence of a finite ferroelectric polarization. The proposed microscopic mechanism is independent of spin-orbit coupling. We predict that the polarization induced by the E-type magnetic order can potentially be enhanced by up to 2 orders of magnitude with respect to that in the spiral magnetic phases of TbMnO3 and similar multiferroic compounds.

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Complexity in strongly correlated electronic systems.

A wide variety of experimental results and theoretical investigations in recent years have convincingly demonstrated that several transition metal oxides and other materials have dominant states that are not spatially homogeneous. This occurs in cases in which several physical interactions-spin, charge, lattice, and/or orbital-are simultaneously active. This phenomenon causes interesting effects, such as colossal magnetoresistance, and it also appears crucial to understand the high-temperature superconductors. The spontaneous emergence of electronic nanometer-scale structures in transition metal oxides, and the existence of many competing states, are properties often associated with complex matter where nonlinearities dominate, such as soft materials and biological systems. This electronic complexity could have potential consequences for applications of correlated electronic materials, because not only charge (semiconducting electronic), or charge and spin (spintronics) are of relevance, but in addition the lattice and orbital degrees of freedom are active, leading to giant responses to small perturbations. Moreover, several metallic and insulating phases compete, increasing the potential for novel behavior.

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Phase fluctuations in strongly coupled d-wave superconductors.

We present a numerically exact solution for the BCS Hamiltonian at any temperature, including the degrees of freedom associated with classical phase, as well as amplitude fluctuations via a Monte Carlo integration. This allows for an investigation over the whole range of couplings: from weak attraction, as in the well-known BCS limit, to the mainly unexplored strong-coupling regime of pronounced phase fluctuations. In the latter, two characteristic temperatures T(*) and T(c), associated with short- and long-range ordering, respectively, can be identified in a mean-field-motivated Hamiltonian. T(*) at the same time corresponds to the opening of a gap in the excitation spectrum. In addition to introducing a novel procedure to study strongly coupled d-wave superconductors, our results indicate that classical phase fluctuations are not sufficient to explain the pseudogap features of high-temperature superconductors.

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Orbital ordering, new phases, and stripe formation in doped layered nickelates.

Ground-state properties of layered nickelates are investigated based on the orbital-degenerate Hubbard model coupled with lattice distortions, by using numerical techniques. The Néel state composed of spin S=1 ions is confirmed in the undoped limit x = 0. At x = 1/2, novel antiferromagnetic states, called CE- and E-type phases, are found by increasing the Hund's coupling. (3x2-r2/3y2-r2)-type orbital ordering is predicted to occur in a checkerboard-type charge-ordered state. At x = 1/3, both Coulombic and phononic interactions are found to be important, since the former stabilizes the spin stripe, while the latter leads to the striped charge order.

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Relevance of cooperative lattice effects and stress fields in phase-separation theories for CMR manganites.

Previous theoretical investigations of colossal magnetoresistance (CMR) materials explain this effect using a "clustered" state with preformed ferromagnetic islands that rapidly align their moments with increasing external magnetic fields. While qualitatively successful, explicit calculations indicate drastically different typical resistivity values in two- and three-dimensional lattices, contrary to experimental observations. This conceptual bottleneck in the phase-separated CMR scenario is resolved here considering the cooperative nature of the Mn-oxide lattice distortions. This effectively induces power-law correlations in the quenched disorder used in toy models with phase competition. When these effects are incorporated, resistor-network calculations reveal very similar results in two and three dimensions, qualitatively modifying previous scenarios and solving the puzzle.

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Unveiling new magnetic phases of undoped and doped manganites.

Novel ground-state spin structures in undoped and lightly doped manganites are investigated based on the orbital-degenerate double-exchange model, via mean-field and numerical techniques. In undoped manganites, a new antiferromagnetic (AFM) state, called the E-type phase, is found adjacent in parameter space to the A-type AFM phase. Its structure is in agreement with recent experimental results. This insulating E-AFM state is also competing with a ferromagnetic metallic phase as well. For doped layered manganites, the phase diagram includes another new AFM phase of the CxE1-x type. Experimental signatures of the new phases are discussed.

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Phase diagram of a model for diluted magnetic semiconductors beyond mean-field approximations.

A lattice spin-fermion model for diluted magnetic semiconductors (DMS) is investigated numerically, improving on previously used mean-field approximations. Curie temperatures are obtained varying the Mn spin x and hole n densities, and the impurity-hole exchange J in units of the hop-ping t. Optimal values are found in the subtle intermediate regime between itinerant and localized carriers. At intermediate and large J/t, a "clustered" state is observed above the Curie temperature and ferromagnetism is suppressed. Formal analogies between DMS and manganites are discussed.

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Prediction of orbital ordering in single-layered ruthenates.

The key role of the orbital degree of freedom to understanding the magnetic properties of layered ruthenates is discussed based on the 3-orbital Hubbard model coupled to lattice distortions, using numerical and mean-field techniques. In the G-type antiferromagnetic phase of Ca(2)RuO(4), recent x-ray experiments reported 0.5 holes/site in the d(xy) orbital, while d(yz) and d(zx) orbitals contain 1.5 holes. This unexpected t(2g) hole distribution is explained by a novel orbital ordered (OO) state, stabilized by a combination of Coulombic and lattice effects. The phase diagram suggests the possibility of large magnetoresistance effects and a new ferromagnetic OO phase in ruthenates.

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