Biomedical subjects

G G Paulus

Publications and source records attributed to G G Paulus.

16 recordsLinked to original sources

PubMed2005

Attosecond double-slit experiment.

A new scheme for a double-slit experiment in the time domain is presented. Phase-stabilized few-cycle laser pulses open one to two windows (slits) of attosecond duration for photoionization. Fringes in the angle-resolved energy spectrum of varying visibility depending on the degree of which-way information are measured. A situation in which one and the same electron encounters a single and a double slit at the same time is observed. The investigation of the fringes makes possible interferometry on the attosecond time scale. From the number of visible fringes, for example, one derives that the slits are extended over about 500 as.

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PubMed2004

Nonsequential double ionization at the single-optical-cycle limit.

We report differential measurements of Ar++ ion momentum distributions from nonsequential double ionization in phase-stabilized few-cycle laser pulses. The distributions depend strongly on the carrier-envelope (CE) phase. Via control over the CE phase one is able to direct the nonsequential double-ionization dynamics. Data analysis through a classical model calculation reveals that the influence of the optical phase enters via (i) the cycle dependent electric field ionization rate, (ii) the electron recollision time, and (iii) the accessible phase space for inelastic collisions. Our model indicates that the combination of these effects allows a look into single cycle dynamics already for few-cycle pulses.

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PubMed2004

Coulomb asymmetry in above-threshold ionization.

A new method for including effects of the Coulomb potential in strong-field laser atom interaction is presented. The model is tested by comparing its results with experimental data of energy resolved angular distributions of photoelectrons. For elliptical polarization these exhibit a strong asymmetry. Our theory shows that this strong asymmetry for the low-energy electrons is induced by a small Coulomb force acting on the tunneling electron just after the exit of the tunnel. This is in contrast to the situation for high electron energies where the asymmetry arises via rescattering by the parent ion.

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PubMed2004

Vortices in femtosecond laser fields.

We experimentally generate optical vortices in the output beam of a 20-fs Ti:sapphire laser. Screw phase dislocations are imposed on the spectral components of the short pulses by aligning a computer-generated hologram in a dispersionless 4f setup.

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PubMed2004

Influence of molecular structure on double ionization of N2 and O2 by high intensity ultrashort laser pulses.

The electron momentum correlation after nonsequential double ionization of N2 and O2 in ultrashort light pulses at light intensities near 1.5 x 10(14) W/cm(2) has been investigated. The experimental results reveal distinctive differences between the molecular species and between molecules and atoms of similar ionization threshold. We provide evidence that recollision double ionization is the essential mechanism and trace the origin of the differences back to the symmetry of the orbitals occupied by the valence electrons.

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PubMed2004

Gouy phase shift for few-cycle laser pulses.

We measured for the first time the influence of the Gouy effect on focused few-cycle laser pulses. The carrier-envelope phase is shown to undergo a smooth variation over a few Rayleigh distances. This result is of critical importance for any application of ultrashort laser pulses, including high-harmonic and attosecond pulse generation, as well as phase-dependent effects.

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PubMed2004

Observation of light-phase-sensitive photoemission from a metal.

We demonstrate that multiphoton-induced photoelectron emission from a gold surface caused by low-energy (unamplified) 4-fs, 750-nm laser pulses is sensitive to the timing of electric field oscillations with respect to the pulse peak. This observation confirms recent theoretical predictions and opens the door to measuring the absolute value of the carrier-envelope phase difference of few-cycle light pulses with a solid-state detector.

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PubMed2003

Measurement of the phase of few-cycle laser pulses.

For the shortest pulses generated to date, the amplitude of the electromagnetic wave changes almost as rapidly as the field oscillates. The temporal variation of the field, which directly governs strong-field interactions, therefore depends on whether the maximum of the pulse amplitude coincides with that of the wave cycle or not, i.e., on the phase of the field with respect to the pulse envelope. It is demonstrated that the direction of electron emission from photoionized atoms can be controlled by varying the phase of the field, providing for the first time a tool for its accurate determination. Directing fast electron emission to the right or to the left with the light phase constitutes a new kind of coherent control.

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PubMed2003

Above-threshold ionization at the few-cycle limit.

Photoelectron spectra measured for rare-gas atoms ionized with intense few-cycle laser pulses are presented. Several aspects of the few-cycle regime are discussed. In particular, the persistence of the plateaulike structure of spectra for high electron energies is shown. In contrast, a resonancelike feature at similar electron energies is suppressed as compared with longer laser pulses. Differences in the behavior of different species and implications for the electron-ion scattering cross section are pointed out.

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PubMed2002

Ring dark solitary waves: experiment versus theory.

Experimental results on optical ring dark solitary wave dynamics are presented, emphasizing the interplay between initial dark beam contrast, total phase shift, background-beam intensity, and saturation of the nonlinearity. The results are found to confirm qualitatively the existing analytical theory and are in agreement with the numerical simulations carried out.

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PubMed2002

Phase-dependent effects of a few-cycle laser pulse.

The Keldysh theory of above-threshold ionization (ATI) is applied to few-cycle laser pulses in order to explore the potential of a recently published new method to measure "carrier-envelope phase difference" phenomena. In this experiment, the carrier-envelope phase difference dependent left-right asymmetry of few-cycle ATI was measured and investigated with a correlation technique. Here, we explore spectral features of the asymmetry, present a theoretical analysis of the experiment, and establish a method to determine the duration of few-cycle pulses whose carrier-envelope phase differences are not controlled.

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PubMed2001

Absolute-phase phenomena in photoionization with few-cycle laser pulses.

Currently, the shortest laser pulses that can be generated in the visible spectrum consist of fewer than two optical cycles (measured at the full-width at half-maximum of the pulse's envelope). The time variation of the electric field in such a pulse depends on the phase of the carrier frequency with respect to the envelope-the absolute phase. Because intense laser-matter interactions generally depend on the electric field of the pulse, the absolute phase is important for a number of nonlinear processes. But clear evidence of absolute-phase effects has yet to be detected experimentally, largely because of the difficulty of stabilizing the absolute phase in powerful laser pulses. Here we use a technique that does not require phase stabilization to demonstrate experimentally the influence of the absolute phase of a short laser pulse on the emission of photoelectrons. Atoms are ionized by a short laser pulse, and the photoelectrons are recorded with two opposing detectors in a plane perpendicular to the laser beam. We detect an anticorrelation in the shot-to-shot analysis of the electron yield.

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PubMed2001

Feynman's path-integral approach for intense-laser-atom interactions.

Atoms interacting with intense laser fields can emit electrons and photons of very high energies. An intuitive and quantitative explanation of these highly nonlinear processes can be found in terms of a generalization of classical Newtonian particle trajectories, the so-called quantum orbits. Very few quantum orbits are necessary to reproduce the experimental results. These orbits are clearly identified, thus opening the way for an efficient control as well as previously unknown applications of these processes.

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PubMed1999

Generation of multiple-charged optical vortex solitons in a saturable nonlinear medium.

Multiply charged optical vortex solitons (OVS) (m=1,...,4) are generated in a thermal nonlinear medium with saturation. The respective soliton constants are found to be linearly proportional to the topological charges. Special attention is paid to the modulational instability, which is effectively suppressed by a moderate saturation but still remains an increasing function of the topological charge. For the particular experimental conditions, the recorded OVS profiles are found to be in good qualitative agreement with the numerical stationary solutions of the generalized nonlinear Schrödinger equation.

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PubMed1999

Modulational instability of multiple-charged optical vortex solitons under saturation of the nonlinearity.

We present a linear analysis and numerical simulations of the instability of optical vortex solitons (OVSs) of arbitrary topological charge. They show a rich variety of instability scenarios depending on the type of perturbation. The saturation of the nonlinearity is shown to be able to slow down the decay of multiple charged dark beams at an intermediate evolution stage and to prevent their ultimate decay into charge-1 OVSs. This concept is experimentally verified by the observation of a partial decay of a triple-charged OV beam and by comparing this dynamic with the behavior of OV beams of topological charges m=1, 2, 3, and 4.

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PubMed1996

A low-cost UV laser for flash photolysis of caged compounds.

Photolysis of caged compounds has become a standard tool for the rapid application of bioactive molecules. In principle this technique also allows to apply substances in a spatially very restricted manner. An important practical limitation for such experiments, however, is the high cost of UV lasers. Here we describe the assembly of an inexpensive pulsed nitrogen laser which is suitable for photolysis experiments. The laser which can be constructed in less than 1 week and for less than US$ 500 emits light pulses with a duration of approximately 5 ns, an energy of up to 200 microJ (= 40 kW) and a wavelength of 337 nm. Its beam can be focused to roughly 30 microns, a firing frequency of up to 50 Hz can be achieved, and electrical artifacts are minimal. These specifications make the laser optimally suited for most photolysis experiments. Its low price and ease of use should make the technique of spatially restricted flash photolysis amenable to many laboratories.

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