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H Walther

Publications and source records attributed to H Walther.

At least 19 recordsLinked to original sources

Attosecond double-slit experiment.

A new scheme for a double-slit experiment in the time domain is presented. Phase-stabilized few-cycle laser pulses open one to two windows (slits) of attosecond duration for photoionization. Fringes in the angle-resolved energy spectrum of varying visibility depending on the degree of which-way information are measured. A situation in which one and the same electron encounters a single and a double slit at the same time is observed. The investigation of the fringes makes possible interferometry on the attosecond time scale. From the number of visible fringes, for example, one derives that the slits are extended over about 500 as.

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Common-mode-free frequency comparison of lasers with relative frequency stability at the millihertz level.

We report on a frequency comparison of frequency-stabilized lasers located in remote laboratories resting on different foundations. By locating the lasers in this way correlated frequency excursions of the lasers are suppressed to a high degree. The beat signal between them shows a linewidth at the hertz level for averaging times of 1 s. The optical link is established by a 100 m single-mode optical fiber where the frequency noise induced by the fiber is reduced to the level of a few tens of millihertz. One laser is stabilized onto a Fabry-Perot resonator with a long-term precision of 25 mHz (fractional frequency instability, sigma(y) = 1.2 x 10(-16)), the highest lock fidelity obtained so far to our knowledge.

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Nonsequential double ionization at the single-optical-cycle limit.

We report differential measurements of Ar++ ion momentum distributions from nonsequential double ionization in phase-stabilized few-cycle laser pulses. The distributions depend strongly on the carrier-envelope (CE) phase. Via control over the CE phase one is able to direct the nonsequential double-ionization dynamics. Data analysis through a classical model calculation reveals that the influence of the optical phase enters via (i) the cycle dependent electric field ionization rate, (ii) the electron recollision time, and (iii) the accessible phase space for inelastic collisions. Our model indicates that the combination of these effects allows a look into single cycle dynamics already for few-cycle pulses.

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How to measure the decoherence of a micromaser field under well controlled conditions.

We discuss a possible realization of a quantum register with controllable decoherence in terms of /0> and /1> photon number states of a micromaser field. It is shown how to create in the Jaynes-Cummings model a superposition state of /0> and /1> photon number states inside a closed micromaser cavity. The loss of phase coherence between these two states can subsequently be measured by a second probe atom monitoring the decoherence of the field. A technique is proposed for forming the superposition of number states /0> and /1> using the time structure of the Rabi oscillation. The proposed method avoids problems with stray fields at the cavity holes, which disturb the coherence of the atomic superposition, and offers a way to study how the coupling strength to the environment influences the decoherence rate, displaying the robustness of physical qubits and the fidelity of quantum computations.

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Vortices in femtosecond laser fields.

We experimentally generate optical vortices in the output beam of a 20-fs Ti:sapphire laser. Screw phase dislocations are imposed on the spectral components of the short pulses by aligning a computer-generated hologram in a dispersionless 4f setup.

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Influence of molecular structure on double ionization of N2 and O2 by high intensity ultrashort laser pulses.

The electron momentum correlation after nonsequential double ionization of N2 and O2 in ultrashort light pulses at light intensities near 1.5 x 10(14) W/cm(2) has been investigated. The experimental results reveal distinctive differences between the molecular species and between molecules and atoms of similar ionization threshold. We provide evidence that recollision double ionization is the essential mechanism and trace the origin of the differences back to the symmetry of the orbitals occupied by the valence electrons.

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Gouy phase shift for few-cycle laser pulses.

We measured for the first time the influence of the Gouy effect on focused few-cycle laser pulses. The carrier-envelope phase is shown to undergo a smooth variation over a few Rayleigh distances. This result is of critical importance for any application of ultrashort laser pulses, including high-harmonic and attosecond pulse generation, as well as phase-dependent effects.

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Measurement of the phase of few-cycle laser pulses.

For the shortest pulses generated to date, the amplitude of the electromagnetic wave changes almost as rapidly as the field oscillates. The temporal variation of the field, which directly governs strong-field interactions, therefore depends on whether the maximum of the pulse amplitude coincides with that of the wave cycle or not, i.e., on the phase of the field with respect to the pulse envelope. It is demonstrated that the direction of electron emission from photoionized atoms can be controlled by varying the phase of the field, providing for the first time a tool for its accurate determination. Directing fast electron emission to the right or to the left with the light phase constitutes a new kind of coherent control.

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Above-threshold ionization at the few-cycle limit.

Photoelectron spectra measured for rare-gas atoms ionized with intense few-cycle laser pulses are presented. Several aspects of the few-cycle regime are discussed. In particular, the persistence of the plateaulike structure of spectra for high electron energies is shown. In contrast, a resonancelike feature at similar electron energies is suppressed as compared with longer laser pulses. Differences in the behavior of different species and implications for the electron-ion scattering cross section are pointed out.

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Fresnel representation of the Wigner function: an operational approach.

We present an operational definition of the Wigner function. Our method relies on the Fresnel transform of measured Rabi oscillations and applies to motional states of trapped atoms as well as to field states in cavities. We illustrate this technique using data from recent experiments in ion traps [Phys. Rev. Lett. 76, 1796 (1996)]] and in cavity QED [Nature (London) 403, 743 (2000)]]. The values of the Wigner functions of the underlying states at the origin of phase space are W(|0>)(0)=+1.75 for the vibrational ground state and W(|1>)(0)=-1.4 for the one-photon number state. We generalize this method to wave packets in arbitrary potentials.

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How to measure the phase diffusion dynamics in the micromaser.

We propose a realistic scheme for measuring the micromaser linewidth by monitoring the phase diffusion dynamics of the cavity field. Our strategy consists of exciting an initial coherent state with the same photon number distribution as the micromaser steady-state field, singling out a purely diffusive process in the system dynamics. After the injection of a counterfield, measurements of the population statistics of a probe atom allow us to derive the micromaser linewidth in all ranges of the relevant parameters, establishing experimentally the distinctive features of the micromaser spectrum due to the discreteness of the electromagnetic field.

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Strong-driving-assisted multipartite entanglement in cavity QED.

We propose a method of generating multipartite entanglement by considering the interaction of a system of N two-level atoms in a cavity of high quality factor with a strong classical driving field. It is shown that, with a judicious choice of the cavity detuning and the applied coherent field detuning, vacuum Rabi coupling produces a large number of important multipartite entangled states. It is even possible to produce entangled states involving different cavity modes. Tuning of parameters also permits us to switch from Jaynes-Cummings to anti-Jaynes-Cummings-like interaction.

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Ring dark solitary waves: experiment versus theory.

Experimental results on optical ring dark solitary wave dynamics are presented, emphasizing the interplay between initial dark beam contrast, total phase shift, background-beam intensity, and saturation of the nonlinearity. The results are found to confirm qualitatively the existing analytical theory and are in agreement with the numerical simulations carried out.

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Absolute-phase phenomena in photoionization with few-cycle laser pulses.

Currently, the shortest laser pulses that can be generated in the visible spectrum consist of fewer than two optical cycles (measured at the full-width at half-maximum of the pulse's envelope). The time variation of the electric field in such a pulse depends on the phase of the carrier frequency with respect to the envelope-the absolute phase. Because intense laser-matter interactions generally depend on the electric field of the pulse, the absolute phase is important for a number of nonlinear processes. But clear evidence of absolute-phase effects has yet to be detected experimentally, largely because of the difficulty of stabilizing the absolute phase in powerful laser pulses. Here we use a technique that does not require phase stabilization to demonstrate experimentally the influence of the absolute phase of a short laser pulse on the emission of photoelectrons. Atoms are ionized by a short laser pulse, and the photoelectrons are recorded with two opposing detectors in a plane perpendicular to the laser beam. We detect an anticorrelation in the shot-to-shot analysis of the electron yield.

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Inhibition of decoherence due to decay in a continuum.

We propose a scheme for slowing down decay into a continuum. We make use of a sequence of ultrashort 2pi pulses applied on an auxiliary transition of the system so that there is a destructive interference between the two transition amplitudes--one before the application of the pulse and the other after the application of the pulse. We give explicit results for a structured continuum. Our scheme can also inhibit unwanted transitions.

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Feynman's path-integral approach for intense-laser-atom interactions.

Atoms interacting with intense laser fields can emit electrons and photons of very high energies. An intuitive and quantitative explanation of these highly nonlinear processes can be found in terms of a generalization of classical Newtonian particle trajectories, the so-called quantum orbits. Very few quantum orbits are necessary to reproduce the experimental results. These orbits are clearly identified, thus opening the way for an efficient control as well as previously unknown applications of these processes.

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Generation of photon number states on demand via cavity quantum electrodynamics.

Many applications in quantum information or quantum computing require radiation with a fixed number of photons. This increased the demand for systems able to produce such fields. We discuss the production of photon fields with a fixed photon number on demand. The first experimental demonstration of the device is described. This setup is based on a cavity quantum electrodynamics scheme using the strong coupling between excited atoms and a single-mode cavity field.

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