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Hanns Walter Müller

Publications and source records attributed to Hanns Walter Müller.

6 recordsLinked to original sources

Ferrofluids as thermal ratchets.

Colloidal suspensions of ferromagnetic nanoparticles, so-called ferrofluids, are shown to be suitable systems to demonstrate and investigate thermal ratchet behavior: By rectifying thermal fluctuations, angular momentum is transferred to a resting ferrofluid from an oscillating magnetic field without net rotating component. Via viscous coupling the noise driven rotation of the microscopic ferromagnetic grains is transmitted to the carrier liquid to yield a macroscopic torque. For a simple setup we analyze the rotation of the ferrofluid theoretically and show that the results are compatible with the outcome of a simple demonstration experiment.

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Thermal convection in binary fluid mixtures with a weak concentration diffusivity, but strong solutal buoyancy forces.

Thermal convection in binary liquid mixtures is investigated in the limit where the solutal diffusivity is weak, but the separation ratio is large. Representative examples are colloidal suspensions such as ferrofluids. With a grain size being large on molecular length scales, the particle mobility is extremely small, allowing to disregard the concentration dynamics in most cases. However, this simplification does not hold for thermal convection: Due to the pronounced Soret effect of these materials in combination with a considerable solutal expansion, the resulting solutal buoyancy forces are dominant. Indeed, convective motion is found to set in at Rayleigh numbers well below the critical threshold for single-component liquids. A nonlinear analysis demonstrates that the amplitude quickly saturates in a state of stationary convective motion.

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Sound damping in ferrofluids: magnetically enhanced compressional viscosity.

The damping of sound waves in magnetized ferrofluids is investigated and shown to be considerably higher than in the nonmagnetized case. This fact may be interpreted as a field-enhanced, effective compressional viscosity-in analogy to the ubiquitous field-enhanced shear viscosity that is known to be the reason for many unusual behaviors of ferrofluids under shear.

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Molecular dynamics study on the equilibrium magnetization properties and structure of ferrofluids.

We investigate in detail the initial susceptibility, magnetization curves, and microstructure of ferrofluids in various concentration and particle dipole moment ranges by means of molecular dynamics simulations. We use the Ewald summation for the long-range dipolar interactions, take explicitly into account the translational and rotational degrees of freedom, coupled to a Langevin thermostat. When the dipolar interaction energy is comparable with the thermal energy, the simulation results on the magnetization properties agree with the theoretical predictions very well. For stronger dipolar couplings, however, we find systematic deviations from the theoretical curves. We analyze in detail the observed microstructure of the fluids under different conditions. The formation of clusters is found to enhance the magnetization at weak fields and thus leads to a larger initial susceptibility. The influence of the particle aggregation is isolated by studying ferro-solids, which consist of magnetic dipoles frozen in at random locations but which are free to rotate. Due to the artificial suppression of clusters in ferrosolids the observed susceptibility is considerably lowered when compared to ferrofluids.

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Shear-excited sound in magnetic fluid.

Perceptible sound is shown to be excited in ferrofluids by the shear motion of a rigid plate, if the fluid is exposed to a magnetic field oblique both to the plate and to the direction of propagation. This is in contrast to other fluids, including anisotropic ones such as nematic liquids.

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