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Hossein Haj-Hariri

Publications and source records attributed to Hossein Haj-Hariri.

3 recordsLinked to original sources

Double-layer thermocapillary convection in a differentially heated cavity.

Many materials-processing applications such as crystal growth from the melt involve thermocapillary flows that can affect the quality of the final product, particularly under microgravity conditions where the influence of buoyancy-driven convection is minimized. When the melt contains volatile components, as in the production of III-V semiconductor crystals, it is often encapsulated in a low-melting point amorphous molten glass phase such as boron oxide or pyrolytic boron nitride in order to prevent evaporation of the volatile components. The addition of the encapsulant layer and the melt-encapsulant interface in such cases can alter the thermocapillary flow in the melt. In this study, thermocapillary convection within a differentially heated rectangular cavity containing two immiscible liquid layers is considered in the absence of gravity. Domain mapping is used in conjunction with a finite difference scheme on a staggered grid to solve for the temperature and flow fields. The melt-encapsulant and the air-encapsulant interfaces are allowed to deform, with the contact lines pinned on the solid boundaries. The computed flow fields are compared to the corresponding results for a cavity with a rigid top surface. The presence of a free surface at the top leads to increased convection in the encapsulant phase while suppressing the thermocapillary flow in the melt phase. The flow pattern in the encapsulated layer is strongly dependent on the viscosity of the encapsulant layer. The intensity of the thermocapillary flow within the melt is significantly reduced as the viscosity of the encapsulant layer is increased. However, for a higher encapsulant viscosity, the retarding effect of the free top surface on thermocapillary convection in the melt is weakened.

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Thermocapillary flow in double-layer fluid structures: an effective single-layer model.

Thermocapillary flows are of considerable technological importance in materials processing applications such as crystal growth from the melt, particularly under microgravity conditions where the influence of buoyancy-driven convection is minimized. In this study, thermally driven convection within a differentially heated rectangular cavity containing two immiscible liquid layers is considered in the absence of gravity. The introduction of a more viscous encapsulant layer leads to a significant reduction in the intensity of the thermocapillary flow within the encapsulated layer. Interface deformations are small when the contact line of the interface is pinned on the solid boundaries. The higher viscosity of the encapsulant layer gives rise to a larger pressure gradient in that layer, thereby resulting in interface deformations that are qualitatively different from those observed at the free surface in the absence of the encapsulant layer. The flow pattern in the encapsulated layer and the resulting interface deformations are strongly dependent on both the thickness and the viscosity of the encapsulant layer. It is shown that the flow within the encapsulated layer may be closely approximated by simply considering the single-layer problem with a modified stress condition at the interface. The modified tangential stress balance for the effective single-layer model is derived based on asymptotic results for small-aspect-ratio double-layer systems and the insight gained from double-layer computations for finite-aspect-ratio systems. It is shown that the single-layer model accurately predicts the flow in the double-layer system even for large aspect-ratios.

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A numerical study of the effect of insoluble surfactants on the stability of a viscous drop translating in a Hele-Shaw cell.

A circular drop is a linearly stable solution for the buoyancy-driven motion of drops in a Hele-Shaw cell [Gupta et al. J. Colloid Interface Sci.218(1), 338 (1999)]. In the absence of surface-active agents, an initially prolate drop always goes to a steady circular shape while initially oblate drops exhibit complex dynamics [Gupta et al. J. Colloid Interface Sci.222, 107 (2000)]. In this study, the effect of insoluble surfactant impurities on the critical conditions for drop breakup is explored by using the Langmuir adsorption framework in conjunction with a physically based expression for the depth-averaged tangential stress exerted on a two-phase interface in a Hele-Shaw cell. It is shown that the presence of surfactants can have both a stabilizing and a destabilizing effect on the shape of the drop, depending on the Bond number, the magnitude of the initial perturbation, and the strength of surface convection. Similar to the clean drop dynamics, two marginally stable branches are found. Increasing the surface Peclet number results in the stabilization of the main branch while the secondary branch shifts to higher Bond numbers. The mode of breakup is also found to be strongly influenced by the strength of surface convection.

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