PubMed Health⌕ Search

Biomedical subjects

I Uschmann

Publications and source records attributed to I Uschmann.

12 recordsLinked to original sources
PubMed2005

High efficiency, high quality x-ray optic based on ellipsoidally bent highly oriented pyrolytic graphite crystal for ultrafast x-ray diffraction experiments.

By the use of a thin highly oriented pyrolytic graphite crystal (HOPG) bent to a high-performance ellipsoidal shape it was possible to focus monochromatic x-rays of 4.5 keV photon energy with an efficiency of 0.0033, which is 30 times larger than for previously used bent crystals. Isotropic Ti K alpha radiation of a 150 microm source was focused onto a 450 microm spot. The size of the focal spot can be explained by broadening due to the mosaic crystal rocking curve. The rocking curve width (FWHM) of the thin graphite foil was determined to 0.11 degrees. The estimated temporal broadening of an ultrashort K alpha pulse by the crystal is not larger than 300 fs. These properties make the x-ray optic very attractive for ultrafast time-resolved x-ray measurements.

Journal Article↗
PubMed2004

High-order Raman scattering of X rays by optical phonons and generation of ultrafast X-ray transients.

We study the modulation of x-ray diffraction in ideal crystals by a copropagating wave of optical vibrations generated by a fs-laser pulse. Our results suggest that in the synchronous interaction regime the output diffracted x-ray field has the form of ultrafast transients with a time structure even shorter than the period of the excited vibrational mode. The behavior is explained in terms of high-order Raman scattering of x rays by optical phonons.

Optics and Photonics↗
PubMed2003

Spatial characteristics of Kalpha x-ray emission from relativistic femtosecond laser plasmas.

The spatial structure of the Kalpha emission from Ti targets irradiated with a high intensity femtosecond laser has been studied using a two-dimensional monochromatic imaging technique. For laser intensities I<5 x 10(17) W/cm(2), the observed spatial structure of the Kalpha emission can be explained by the scattering of the hot electrons inside the solid with the help of a hybrid particle-in-cell/Monte Carlo model. By contrast, at the maximum laser intensity I=7 x 10(18) W/cm(2) the half-width of the Kalpha emission was 70 microm compared to a laser-focus half-width of 3 microm. Moreover, the main Kalpha peak was surrounded by a halo of weak Kalpha emission with a diameter of 400 microm and the Kalpha intensity at the source center did not increase with increasing laser intensity. These three features point to the existence of strong self-induced fields, which redirect the hot electrons over the target surface.

Journal Article↗
PubMed2002

Optimization of Kalpha bursts for photon energies between 1.7 and 7 keV produced by femtosecond-laser-produced plasmas of different scale length.

The conversion efficiency of a 90 fs high-power laser pulse focused onto a solid target into x-ray Kalpha line emission was measured. By using three different elements as target material (Si, Ti, and Co), interesting candidates for fast x-ray diffraction applications were selected. The Kalpha output was measured with toroidally bent crystal monochromators combined with a GaAsP Schottky diode. Optimization was performed for different laser intensities as well as for different density scale lengths of a preformed plasma. These different scale lengths were realized by prepulses of different intensities and delay times with respect to the main pulse. Whereas the Kalpha yield varied by a factor of 1.8 for different laser intensities, the variation of the density scale length could provide a gain factor up to 4.6 for the Kalpha output.

Journal Article↗
PubMed2002

Theory of K(alpha) generation by femtosecond laser-produced hot electrons in thin foils.

An analytical model of femtosecond K(alpha) x-ray generation from laser-irradiated foils is presented. Expressions are found for the photon emission yield in both forward and backward directions in integral form as a function of hot-electron temperature and target thickness. It is found that for any given target material, there is a foil thickness and a hot-electron temperature at which the K(alpha) emission is maximized. Conversion efficiencies are consistent with contemporary measurements of K(alpha) radiation produced with femtosecond lasers.

Journal Article↗
PubMed2002

Spectroscopic determination of dynamic plasma gradients in implosion cores.

The time-dependent gradient structure of a laser-compressed, high-energy-density plasma has been determined using a method based on the simultaneous analysis of time-resolved x-ray monochromatic images and x-ray line spectra from Ar-doped D2 implosion cores. The analysis self-consistently determines the temperature and density gradients that yield the best fits to the spatial-emissivity profiles and spectral line shapes. This measurement is important for understanding the spectra formation and plasma dynamics associated with the implosion process. In addition, since the results are independent of hydrodynamic simulations, they are also important for comparison with fluid-dynamic models.

Journal Article↗
PubMed2001

Femtosecond silicon K alpha pulses from laser-produced plasmas.

Ultrashort bursts of silicon K alpha x-ray radiation from femtosecond-laser-produced plasmas have been generated. A cross-correlation measurement employing a laser-triggered ultrafast structural change of a CdTe crystal layer (320 nm) shows a K alpha pulse duration between 200 fs and 640 fs. This result is corroborated by particle in cell simulations combined with a Monte-Carlo electron stopping code and calculations on the structural changes of the crystal lattice.

Journal Article↗
PubMed2001

Non-thermal melting in semiconductors measured at femtosecond resolution.

Ultrafast time-resolved optical spectroscopy has revealed new classes of physical, chemical and biological reactions, in which directed, deterministic motions of atoms have a key role. This contrasts with the random, diffusive motion of atoms across activation barriers that typically determines kinetic rates on slower timescales. An example of these new processes is the ultrafast melting of semiconductors, which is believed to arise from a strong modification of the inter-atomic forces owing to laser-induced promotion of a large fraction (10% or more) of the valence electrons to the conduction band. The atoms immediately begin to move and rapidly gain sufficient kinetic energy to induce melting--much faster than the several picoseconds required to convert the electronic energy into thermal motions. Here we present measurements of the characteristic melting time of InSb with a recently developed technique of ultrafast time-resolved X-ray diffraction that, in contrast to optical spectroscopy, provides a direct probe of the changing atomic structure. The data establish unambiguously a loss of long-range order up to 900 A inside the crystal, with time constants as short as 350 femtoseconds. This ability to obtain the quantitative structural characterization of non-thermal processes should find widespread application in the study of ultrafast dynamics in other physical, chemical and biological systems.

Journal Article↗
PubMed2000

Yield optimization and time structure of femtosecond laser plasma kalpha sources

The generation of femtosecond Kalpha x rays from laser-irradiated plasmas is studied with a view to optimizing photon number and pulse duration. Using analytical and numerical models of hot electron generation and subsequent transport in a range of materials, it is shown that an optimum laser intensity I(opt) = 7x10(9)Z4.4 exists for maximum Kalpha yield. Furthermore, it is demonstrated that bulk targets are unsuitable for generating sub-ps x-ray pulses: instead, design criteria are proposed for achieving Kalpha pulse durations </=100 fs using foils of approximately 2 &mgr;m thickness.

Journal Article↗