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J Handl

Publications and source records attributed to J Handl.

17 recordsLinked to original sources

Ant-based clustering and topographic mapping.

Ant-based clustering and sorting is a nature-inspired heuristic first introduced as a model for explaining two types of emergent behavior observed in real ant colonies. More recently, it has been applied in a data-mining context to perform both clustering and topographic mapping. Early work demonstrated some promising characteristics of the heuristic but did not extend to a rigorous investigation of its capabilities. We describe an improved version, called ATTA, incorporating adaptive, heterogeneous ants, a time-dependent transporting activity, and a method (for clustering applications) that transforms the spatial embedding produced by the algorithm into an explicit partitioning. ATTA is then subjected to the most rigorous experimental evaluation of an ant-based clustering and sorting algorithm undertaken to date: we compare its performance with standard techniques for clustering and topographic mapping using a set of analytical evaluation functions and a range of synthetic and real data collections. Our results demonstrate the ability of ant-based clustering and sorting to automatically identify the number of clusters inherent in a data collection, and to produce high quality solutions; indeed, we show that it is particularly robust for clusters of differing sizes and for overlapping clusters. The results obtained for topographic mapping are, however, disappointing. We provide evidence that the solutions generated by the ant algorithm are barely topology-preserving, and we explain in detail why results have--in spite of this--been misinterpreted (much more positively) in previous research.

Algorithms↗

Iodine-129 in soils from Northern Ukraine and the retrospective dosimetry of the iodine-131 exposure after the Chernobyl accident.

Forty-eight soil profiles down to a depth of 40 cm were taken in Russia and Ukraine in 1995 and 1997, respectively, in order to investigate the feasibility of retrospective dosimetry of the 131I exposure after the Chernobyl accident via the long-lived 129I. The sampling sites covered areas almost not affected by fallout from the Chernobyl accident such as Moscow/Russia and the Zhitomir district in Ukraine as well as the highly contaminated Korosten and Narodici districts in Ukraine. 129I was analyzed by radiochemical neutron activation analysis (RNAA) and accelerator mass spectrometry (AMS). 127I was measured for some profiles by RNAA or ion chromatography (IC). The results for 127I demonstrated large differences in the capabilities of the soils to store iodine over long time spans. The depth profiles of 129I and of 137Cs showed large differences in the migration behavior between the two nuclides but also for each nuclide among the different sampling sites. Though it cannot be quantified how much 129I and 137Cs was lost out of the soil columns into deeper depths, the inventories in the columns were taken as proxies for the total inventories. For 129I, these inventories were at least three orders of magnitude higher than a pre-nuclear value of 0.084+/-0.017 mBq m(-2) derived from a soil profile taken in 1939 in Lutovinovo/Russia. From the samples from Moscow and Zhitomir, a pre-Chernobyl 129I inventory of (44+/-24) mBq m(-2) was determined, limiting the feasibility of 129I retrospective dosimetry to areas where the 129I inventories exceed 100 mBq m(-2). Higher average 129I inventories in the Korosten and Narodici districts of 130 and 848 mBq m(-2), respectively, allowed determination of the 129I fallout due to the Chernobyl accident. Based on the total 129I inventories and on literature data for the atomic ratio of 129I/131I=13.6+/-2.8 for the Chernobyl emissions and on aggregated dose coefficients for 131I, the thyroid exposure due to 131I after the Chernobyl accident was estimated for the inhabitants of four villages in the Korosten and of three villages in the Narodici districts. The limitations and uncertainties of the 129I retrospective dosimetry are discussed.

Chernobyl Nuclear Accident↗

Evaluation of radioactive exposure from 137Cs in contaminated areas of Northern Ukraine.

The paper gives averages of 137Cs deposition densities in soils from three areas in Northern Ukraine measured 12 to 15 y following the Chernobyl accident: in an area near Narodici (75 km west of the Chernobyl nuclear power plant in the so-called zone II) heavily contaminated by the Chernobyl fall-out and in areas around Korosten and Zhitomir showing contamination levels to be much lower. The three areas exhibited very different 137Cs deposition densities of 2.2 MBq m(-2), 400 kBq m(-2), and 5 kBq m(-2), respectively. During a 1-y observation, measurements of the 137Cs transfer in the food chain to humans and 137Cs whole body contents dependent on the 137Cs daily intake were carried out under realistic conditions of the rural inhabitants who lived in settlements within zone II. Detailed investigations of components of the daily diet showed that the high 137Cs contamination levels found in soils of zone II do not affect in any way low 137Cs concentrations of all important agricultural products harvested and consumed by villagers. With regard to consumption habits of the population of zone II, mushrooms and wild berries were found to contribute more than 95% of the 137Cs daily intake to the 137Cs whole body content of about 12 kBq (with maximum values up to 760 kBq) measured in a group of inhabitants of zone II during a period from July 1998 to July 1999. The median of the annual dose of these inhabitants from external and internal exposures was 1.2 mSv y(-1) with a geometric standard deviation of 2.6. Excluding extreme habits, the geometric mean of the total exposure was 1.0 mSv y(-1) with a geometric standard deviation of 1.3.

Adolescent↗

Fallout radiocesium in an Antarctic region: deposition history, activity densities and vertical transport in soils.

To improve the knowledge about the (137)Cs spatial distribution and vertical migration in soils of the Southern Hemisphere, the total areal activity density and the vertical transport parameters of this radionuclide were measured in an Antarctic region. For this purpose vegetation and incremental soil samples were collected at 21 representative sites located at 4 islands of the South Shetland Archipelago: King George, Robert, Greenwich and Snow (62-63 degrees S and 58-62 degrees W). The total (137)Cs activity density varied considerably from 118 to 662 Bq m(-2) (median 384 Bq m(-2), reference date 1995), with a high percentage of the total activity retained in the vegetation cover (5-98% in moss, 3-20% in lichen and 4-12% in grass). At most sites, the maximum activity density in soil was observed in the top layer from where it decreased continuously. To evaluate the transport parameters of (137)Cs from the activity-depth profiles, the classical convection-diffusion model was used based on the time-course of the annual deposition density of (137)Cs at the studied region. The values for the diffusion coefficient D(s) (median 0.043 cm(2) year(-1)) and the convection velocity v(s) (median -0.012 cm year(-1)) of radiocesium observed under a polar climate are small compared to the transport parameters determined in temperate zones. The data also indicate that at these sites the convectional transport of (137)Cs is almost negligible compared to the transport by diffusion. The high vulnerability of the Antarctic soils to (137)Cs deposition, as a consequence of its very slow transport due to the extreme climatic conditions at these latitudes, has been confirmed.

Antarctic Regions↗

Global weapons' fallout 137Cs in soils and transfer to vegetation in south-central Chile.

The contamination and depth distribution of 137Cs in soil due to the fallout from atmospheric weapons' tests were measured at 29 sites in the 9th and 10th administrative regions in Chile located in the 40 degrees latitude in the southern hemisphere. The depth distribution in most of the sites follows no systematic pattern in the upper few centimetres, but below this depth an exponential decline could be deduced. The calculated relaxation depth appears to be a good indicator for estimating the long-term 137Cs distribution in these soil profiles. It ranges from 4.4 +/- 1.9 cm in Palehumults to 8.4 +/- 4.4 and 9.7 +/- 5.1 cm in Hapludands and Psamments, respectively. For these soil types the value for the relaxation depth tends to increase with decreasing clay content and increasing volume of coarse pores. 137Cs activity densities at the selected sites ranged from 450 to 5410 Bq m(-2) and correlate significantly (r = 0.791) with the mean annual rainfall rate of the sampling sites. 137Cs concentration ratios of prairie plants/soil were found to be in the range 0.008-2.3 and could be related to relaxation depths in undisturbed soils.

Cesium Radioisotopes↗

On the analysis of iodine-129 and iodine-127 in environmental materials by accelerator mass spectrometry and ion chromatography.

Based on a review of literature about the abundances of 129I (T1/2 = 15.7 Ma) in the environment we show that there is a severe lack of knowledge, in particular about natural, pre-nuclear levels. Among the two analytical techniques which are sensitive enough to investigate 129I in environmental materials, namely radiochemical neutron activation analysis (RNAA) and accelerator mass spectrometry (AMS), only AMS is capable of covering the natural, pre-nuclear levels. Since such AMS measurements require chemical separation of iodine from the matrix, a wide variety of separation schemes are necessary for environmental analyses. We report here on such schemes for the analysis of soils, plants and soft tissue. They are applied exemplarily to analyses of soils from the vicinity of Chernobyl. For chemical separations prior to analysis, contamination control and blank analyses are essential. Here, we discuss quality control procedures in detail, both for RNAA and AMS. In the case of AMS we use ion-chromatography (IC) for the determination of stable iodine. The IC analysis is included in the separation schemes for environmental materials. First AMS-analyses of terrestrial biospheric materials demonstrate that natural environmental levels of 129I are lower than previously deduced from investigations using RNAA, but higher than expected from model calculations. AMS is capable of providing the missing knowledge about the radioecology of 129I.

Air Pollutants, Radioactive↗

Long-term decrease of atmospheric test 137Cs in the soil-prairie plant-milk pathway in southern Chile.

The time dependency of nuclear test 137Cs in soil, prairie plants, and milk was observed on pastures of seven dairy farms in the 10th Region, Chile, from 1982 to 1997, without any appreciable deposition of radioactive fallout after 1983. Whereas the 137Cs concentration in the soil decreased at a rate close to that of the radionuclide's physical decay during the whole observation period, the rate of decrease of the 137Cs concentration in the prairie plants and in the milk, having been very rapid between 1982-1990, became slower between 1991-1997. The effective half-lives of the concentration in plants were found to be 5.6 y and 12 y during the first and second observation periods, respectively. Similar half-lives of 5.5 y and 13 y were found for the concentration decline in milk during each period. These data clearly demonstrate a reduction in the long-term decrease of the 137Cs plant uptake, and consequently in the decrease of the 137Cs concentration in milk, resulting from a decline of 137Cs availability for prairie plants in the Hapludand soils over the whole 15-y observation period.

Animals↗

129I, 131I and 127I in animal thyroids after the Chernobyl nuclear accident.

A small number of animal thyroids from Bad Hall, Austria; Ulm, Germany; and Steinkjer, Norway had 131I (half-life 8.06 d) measured between 21 and 72 d following the nuclear accident at Chernobyl on 26 April 1986. Nine years later 129I (half-life 1.57 x 10(7) y) fission product and natural 127I were measured in the same thyroids. The mass ratios, 129I/131I were calculated to the date of the Chernobyl accident and they ranged between 13 and 71. These ratios are compared to the expected ratios within an operating nuclear reactor during 2 y of operation, where the 129I/131I(-1) ratio never exceeded 30. The observed ratio of 129I to natural 127I in thyroids ranged from 5 to 200 times the ratio before the accident, except that the Norwegian thyroids had 129I/127I ratios which were less than the ratios of pre-Chernobyl thyroids from Ulm. These studies show the 129I and 131I from the Chernobyl accident were accumulated with natural 127I in animal thyroids but the isotope ratios, calculated to the release date, had wide ranges. The 131I radioactive exposure might be estimated from a fission product mixture by measuring 129I in thyroids long after the exposure to 131I, but the results would probably show a wide range of possibilities. The determining variables should be evaluated. We know of no previous data regarding both 131I and 129I in thyroid glands during the first 3 mo after the Chernobyl accident.

Animals↗

137Cs concentration in soil, prairie plants, and milk from sites in southern Chile.

Soil, prairie plants, and milk samples were collected at 39 dairy farms in the 9th and 10th Region in Southern Chile (38 degrees 44'-41 degrees 08' S) between 1982 and 1990. 137Cs concentrations found in soil, plant, and milk samples ranged from 3.8-17.1 Bq kg-1 for soil, from < 0.3-20 Bq kg-1 dry mass for plants, and from 0.10-0.71 Bq kg-1 for milk. Cesium concentration levels resulting from soil sample measurements exhibit a close similarity with corresponding values found in soils from Central Europe before 1986. The concentration ratio prairie plants:soil ranged from 0.05-0.62, 0.52-5.0, and < 0.02-0.40 corresponding to Dystrandepts, Placandepts, and Palehumults soil groups, respectively. At seven selected dairy farms in the vicinity of Valdivia city (10th Region), soil, prairie plant, and milk samples were taken yearly during the grazing period between 1982 and 1990. Results obtained from soil samples taken after April 1986 show no significant increase of the 137Cs concentration. Concentrations in plants and milk for 137Cs decreased during the observation time. 134Cs (as an indicator of Chernobyl fallout) was not found in soil, plant, or milk samples during 1986-1990.

Animals↗

Biospheric 129I concentrations in the pre-nuclear and nuclear age.

In order to detect characteristic regional differences or temporal changes of 129I concentrations in the biosphere, thyroids from humans, grazing livestock, and herbivorous wildlife species (reindeer and roedeer) were collected in various areas of the world which are not affected by reprocessing plants. For reasons of comparison, all samples were analyzed for their 129I:127I atom ratios. Human and bovine thyroids taken from the 10th region in Southern Chile (39 degrees-41 degrees South) indicated values of the 129I:127I atom ratio between 1.1 x 10(-9) and 2.0 x 10(-9) and between 1.2 x 10(-10) and 9 x 10(-9), respectively. They showed no significant increase in the concentration of biospheric 129I in comparison with that established in the pre-nuclear age. Atom ratios found in human thyroids collected in Lower Saxony (Federal Republic of Germany), which is a region not directly affected by reprocessing plants, exhibited 129I:127I values between 8 x 10(-9) and 6 x 10(-8) from February 1988 to September 1990. Thyroid glands of reindeer and roedeer as well as heather, moss, and lichen were taken from the Vilhelmina, Heby, and Gävle communes in Sweden and analyzed for 129I and 127I. All three communes were found to be seriously contaminated by fallout from the Chernobyl accident. Highest 129I:127I atom ratios between 3.5 x 10(-7) and 1 x 10(-6) were found in the Gävle commune (approximately 150 km northwest of Stockholm) where the highest 137Cs ground deposition (70-80 kBq m-2) was measured. Two soil samples taken from Krasnaya Gora and Mirny locations in Russia (approximately 200 km northeast of Chernobyl) exhibited ratios of about 1 x 10(-6). These locations showed a 137Cs ground deposition of 370 and 1,300 kBq m-2, respectively.

Animals↗

Measurements of 129I in human and bovine thyroids in Europe--transfer of 129I into the food chain.

Bovine thyroid glands from different countries in Europe and human thyroid glands from Lower Saxony (Federal Republic of Germany) show isotopic 129I/127I ratios of 2.1 X 10(-9) to 8.2 X 10(-8) for cattle and 2.1 X 10(-9) to 8 X 10(-8) in humans. These values give information about the concentration of fallout 129I in Europe since most of these glands were collected in areas without nuclear facilities. Some of the human thyroids were collected after the Chernobyl accident between May 1986 and February 1988. Results obtained from human thyroids taken in some locations of Lower Saxony show no significant increase of the 129I during this time. Higher concentrations of 129I were only found in cattle grazing in the vicinity of a reprocessing plant in Mol, Belgium. Samples of soil, vegetation, milk, and water from this area contained higher than normal concentrations of 129I. The long-term transfer of radioiodine from the soil to the plant and the translocation within the soil were studied using a soil monolith with a 129I-contaminated surface. During the 4 y of the experiment, the transfer factor plant/soil decreased from 0.3 to 2.2 X 10(-3). Soil samples taken in 5-cm steps to a depth of 30 cm then at 40 and 50 cm depths showed that the transport of radioiodine to lower layers proceeds very slowly. The top 5-cm layer contained about 80% of the total radioactivity 52 mo after contamination. In an in-vivo study with a dairy cow, the transfer of radioiodine from feed to milk to cow meat and to pig thyroid gland was followed for 53 d using 129I-labeled pasture grass contaminated via roots. A part of the milk obtained from the cow was fed to a pig as a substitute for humans. The mean value of the transfer factor milk/feed was 2.4 X 10(-3) d kg-1. The values of the transfer factor cow meat/feed obtained for different muscle cuts and organs (excluding thyroid) ranged between 3.0 X 10(-4) (kidney) and 5.4 X 10(-2) d kg-1 f.w. The transfer factors pig thyroid/milk (as pig feed) and pig thyroid/cow feed exhibited values of 1.2 and 8.7 X 10(-3) d kg-1 f.w., respectively.

Animal Feed↗

Long-term transfer of I-129 into the food chain.

To investigate the transfer of Iodine-129 along the feed-animal-milk-pig thyroid pathway under conditions of short- and long-term contamination, two feeding experiments with dairy cows were carried out. Pasture grass radiolabelled with I-129 via root uptake was used as labelled feed in both experiments. During the first experiment the transfer of I-129 from feed to milk and the effective removal half-life of I-129 in the milk were determined after constant doses of I-129 in the labelled grass had been administered for a period of 8 days. In the second experiment the long term transfer of I-129 from feed-to-milk-to-cow-meat and to pig thyroid gland was followed for a period of 53 days. The pig was used because of the physiological similarity between pigs and humans. The effective half-life for removal of I-129 from milk was found to be 1.6 days. The values for the transfer factor from feed-to-milk (in units of day kg-1) resulting from the 1st assay ranged between 1.0.10(-3) and 1.7.10(-3). The long term feeding experiment exhibited a middle value for the transfer factor of 2.4.10(-3). The transfer factors pig thyroid/milk (as pig feed) and pig thyroid/cow feed exhibited values of 1.2 and 8.7.10(-3) respectively.

Animal Feed↗

Transfer from soil to plants of 106Ru as nitrosyl and as chloride.

The transfer of 106Ru in a soil-plant ecosystem was investigated with respect to two chemical forms in compact soil samples under greenhouse conditions with surface and deep-layer contamination. Considerable differences in the uptake of 106Ru were observed between 106RuCl3 and 106Ru-nitrosyl during the first 5-8 wk after the contamination of the soil. The translocation of 106Ru in the soil showed an inhomogeneous distribution of the radioruthenium, with a great part of the total activity remaining in the upper soil layer between 0 and 5 cm even 10 mo after contamination of the soil surface. During the whole experiment, reemission of 106Ru into the air was investigated by using special air collectors under different temperature and light conditions. Although a continuous checking out for a time of about 8 mo, no measurable concentrations of 106Ru could be out for a time of about 8 mo, no measurable concentrations of 106Ru could be found in examined air filters.

Plants↗

Content and heterogeneity of distribution of iodine in human and bovine thyroid glands determined by neutron activation analyses.

While performing activation analytical investigations on the actual concentration of the long-lived radioactive 129iodine in human and bovine thyroid glands the absolute natural nonradioactive 127 iodine content was determined. In all thyroid glands an uneven distribution of 127I was found (in human thyroids from 0 to 0.75 micrograms 127I /mg, in bovine thyroids from 0 to 3.5 micrograms 127I /mg). The mean value of iodine concentration in human thyroid glands ranged from 230 micrograms/g to 490 micrograms/g. This is important because TSH independent autonomy is found at a cellular and follicular level during the development from diffuse to nodular goiter. Both processes may, however, not be related to each other. The resolution of the method used in our study is between the microscopic and the scintigraphic level with an accuracy of +/- 1%, and it shows an intermediate heterogeneity of iodine in thyroid glands.

Adult↗

The influence of soil parameters on 137Cs+-uptake by plants from long-term fallout on forest clearings and grassland.

An attempt was made to show if and to what extent the 137Cs transfer from soil to plants (grass) in forest clearings and grassland is related closely enough to different soil parameters to make it worthwhile to develop mathematical models for the prediction of transfer coefficients for certain plants and sites based solely on soil parameters. For this reason 62 soil samples from 0- to 5-cm in depth as well as from 5- to 10-cm in depth were measured for worldwide 137Cs fallout and analyzed for exchangeable potassium content, total potassium content, clay fraction, potential exchange capacity, pH value and carbon content. For both ecosystems, large variations of the transfer coefficients were observed: between 0.01 and 0.1 for grassland and 0.05 and 6 for forest clearings . Correlations, such as has been found between soil parameters, specific activities of the plants and transfer coefficients can in principle be integrated into different calculations for the estimation of radiation burden.

Cesium Radioisotopes↗