PubMed Health⌕ Search

Biomedical subjects

J L García-Palacios

Publications and source records attributed to J L García-Palacios.

2 recordsLinked to original sources

Spin dynamics in a dissipative environment: from quantal to classical.

We address the problem of spin dynamics in the presence of a thermal bath, by solving exactly the appropriate quantum master equations with continued-fraction methods. The crossover region between the quantum and classical domains is studied by increasing the spin value , and the asymptote for the classical absorption spectra is eventually recovered. Along with the recognized relevance of the coupling strength, we show the critical role played by the structure of the system-environment interaction in the emergence of classical phenomenology.

Journal Article↗

Large quantum nonlinear dynamic susceptibility of single-molecule magnets.

The nonlinear dynamical response of Mn12 single-molecule magnets is experimentally found to be very large, quite insensitive to the spin-lattice coupling constant, and displaying peaks reversed with respect to classical superparamagnets. It is shown that these features are caused by the strong field dependence of the relaxation rate due to the detuning of energy levels between which tunneling takes place. The nonlinear susceptibility technique, previously overlooked, is thus proposed as a privileged probe to ascertain the occurrence of quantum effects in mesoscopic magnetic systems.

Journal Article↗