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J van Duijn

Publications and source records attributed to J van Duijn.

5 recordsLinked to original sources
PubMed2006

Metallic spin-liquid behavior of the geometrically frustrated Kondo lattice.

Strongly frustrated magnetism of the metallic pyrochlore oxide Pr2Ir2O7 has been revealed by single crystal study. While Pr 4f moments have an antiferromagnetic RKKY interaction energy scale of /T*/ = 20 K mediated by Ir 5d-conduction electrons, no magnetic long-range order is found except for partial spin freezing at 120 mK. Instead, the Kondo effect, including a lnT dependence in the resistivity, emerges and leads to a partial screening of the moments below /T*/. Our results indicate that the underscreened moments show spin-liquid behavior below a renormalized correlation scale of 1.7 K.

Journal Article↗
PubMed2005

Inhomogeneous level splitting in Pr 2-x BixRu2O7.

We report that Bi doping drives Pr 2-x BixRu2O7 from an antiferromagnetic insulator (x = 0) to a metallic paramagnet (x approximately 1) with a broad low T maximum in C/T. Neutron scattering reveals local low energy spin excitations (variant Planck's omega approximately 1 meV) with a spectrum that is unaffected by heating to k(B)T >> variant Planck's omega. We show that a continuous distribution of splittings of the non-Kramers Pr3+ ground-state doublet such as might result from various types of lattice strain can account for all the data.

Journal Article↗
PubMed2004

Random fields and the partially paramagnetic state of CsCo0.83Mg0.17Br3: critical scattering study.

We have performed measurements of the critical neutron scattering on CsCo0.83Mg0.17Br3, a dilute stacked triangular lattice (STL) Ising antiferromagnet (AF). A two component line shape associated with the critical fluctuations appears at a temperature coincident with T(N1) observed in pure CsCoBr3. Such scattering is indicative of fluctuations in prototypical random field Ising model (RFIM) systems. The random field domain state arises in this case due to geometrical frustration within the STL Ising AF, which gives rise to a three sublattice Néel state, in which one sublattice is disordered. Magnetic vacancies nucleate AF domains in which the vacancies reside on the disordered sublattice thereby generating a RFIM state in the absence of an applied magnetic field.

Journal Article↗
PubMed2003

Unconventional magnetic correlations in DyB2C and HoB2C.

Layered borocarbides RB2C (R=Dy, Ho, and Er) have been studied by powder neutron diffraction at 2-30 K. ErB2C has two-sublattice antiferromagnetic order below T(N)=16.3 K, but DyB2C and HoB2C show a coexistence of a conventional canted k=(000) ferromagnetic structure and unconventional magnetic correlations. The k=(000) phase orders at T(c)=8.5 K (DyB2C) and 7.1 K (HoB2C), but low-Q diffraction peaks from the unconventional correlations appear above T(c) with different critical temperatures for different peaks: at 8, 10.5, and 15.7 K for HoB2C. This scattering is fitted as diffraction from a Warren-type random magnetic layer lattice and may result from quadrupolar interactions between R3+ spins.

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