Surface plasmon resonances of free-standing gold nanowires fabricated by nanoskiving.
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Biomedical subjects
Publications and source records attributed to Jiming Bao.
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We report a hybrid approach for photonic systems that combines chemically synthesized single nanowire emitters with lithographically defined photonic crystal and racetrack microresonator structures. Finite-difference time-domain calculations were used to design nanowire photonic crystal structures where the photonic band gap overlaps the electronic band gap of the nanowire. Photoluminescence (PL) images of cadmium sulfide (CdS) nanowire photonic crystal structures designed in this way demonstrate localized emission from engineered defects and light suppression in regions of the photonic crystal. PL spectroscopy studies of defect-free nanowire photonic crystal structures further demonstrate the photonic band gap or stop band that spans most of the CdS band edge emission spectrum. In addition, single CdS nanowire-racetrack microresonator structures were fabricated, and PL imaging and spectroscopy measurements show good coupling of the nanowire to the microcavity including efficient feedback and amplified spontaneous emission. These hybrid structures exploit unique strengths of bottom-up and top-down approaches and thereby open new opportunities in nanophotonics from efficient and localized light sources to integrated optical processing.
We present a novel technique for reliable electrical injection into single semiconductor nanowires for light-emitting diodes and lasers. The method makes use of a high-resolution negative electron-beam resist and direct electron-beam patterning for the precise fabrication of a metallic top contact along the length of the nanowire, while a planar substrate is used as a bottom contact. It can be applied to any nanowire structure with an arbitrary cross section. We demonstrate this technique by constructing the first zinc oxide single-nanowire light-emitting diode. The device exhibits broad sub-bandgap emission at room temperature.
According to quantum mechanics, a many-particle system is allowed to exhibit non-local behaviour, in that measurements performed on one of the particles can affect a second one that is far away. These so-called entangled states are crucial for the implementation of most quantum information protocols and, in particular, gates for quantum computation. Here we use ultrafast optical pulses and coherent techniques to create and control spin-entangled states in an ensemble of non-interacting electrons bound to donors (at least three) and at least two Mn2+ ions in a CdTe quantum well. Our method, relying on the exchange interaction between localized excitons and paramagnetic impurities, can in principle be applied to entangle an arbitrarily large number of spins.