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L Limot

Publications and source records attributed to L Limot.

4 recordsLinked to original sources

Atom transfer and single-adatom contacts.

The point contact of a tunnel tip approaching towards Ag(111) and Cu(111) surfaces is investigated with a low temperature scanning tunneling microscope. A sharp jump to contact, random in nature, is observed in the conductance. After point contact, the tip-apex atom is transferred to the surface, indicating that a one-atom contact is formed during the approach. In sharp contrast, the conductance over single silver and copper adatoms exhibits a smooth and reproducible transition from tunneling to contact regime. Numerical simulations show that this is a consequence of the additional dipolar bonding between the adatom and the surface atoms.

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Surface-state localization at adatoms.

Low-temperature scanning tunneling spectroscopy of magnetic and nonmagnetic metal atoms on Ag(111) and on Cu(111) surfaces reveals the existence of a common electronic resonance at an energy below the binding energies of the surface states. Using an extended Newns-Anderson model, we assign this resonance to an adsorbate-induced bound state, split off from the bottom of the surface-state band, and broadened by the interaction with bulk states. A line shape analysis of the bound state indicates that Ag and Cu adatoms on Ag(111) and Cu(111), respectively, decrease the surface-state lifetime, while a cobalt adatom causes no significant change.

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Surface-state Stark shift in a scanning tunneling microscope.

We report a quantitative low-temperature scanning tunneling spectroscopy (STS) study on the Ag(111) surface state over an unprecedented range of currents (50 pA to 6 microA) through which we can tune the electric field in the tunnel junction of the microscope. We show that in STS a sizable Stark effect causes a shift of the surface-state binding energy E0. Data taken are reproduced by a one-dimensional potential model calculation, and are found to yield a Stark-free energy E0 in agreement with recent state-of-the-art photoemission spectroscopy measurements.

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Ga NMR study of the local susceptibility in Kagome-based SrCr8Ga4O19: pseudogap and paramagnetic defects

We present the first Ga(4f ) NMR study of the Cr susceptibility in the archetype of kagome-based frustrated antiferromagnets, SrCr8Ga4O19. Our major finding is that the susceptibility of the frustrated lattice goes through a maximum around 50 K. Our data also support the existence of paramagnetic "clusters" of spins, responsible for the Curie behavior observed in the macroscopic susceptibility at low T. These results set novel features for the constantly debated physics of geometrically frustrated magnets.

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