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Limin Zeng

Publications and source records attributed to Limin Zeng.

4 recordsLinked to original sources

Source apportionment of PM2.5 in Beijing in 2004.

Based on measurements of fine particulate matter (PM2.5, i.e., particles with an aerodynamic diameter of 2.5 microm or less) in January and August 2004, serious air pollution persists in Beijing. The chemical analysis included organic and elemental carbon, water-soluble ions, and elemental compositions. The positive matrix factorization (PMF) method was used to apportion the PM2.5 sources. The sources contributing dominantly to PM2.5 mass concentrations are coal combustion in winter and the secondary products in summer. Furthermore, the contributions from motor vehicles, road dusts and biomass burning could not be neglected. The products of biomass burning for winter heating in the area around Beijing could enter the urban area during quasi-quiescent weather conditions. In conclusion, some effective control measures were proposed to reduce the PM2.5 pollution in Beijing.

Air Pollutants↗

Source apportionment of PM2.5 in Beijing using principal component analysis/absolute principal component scores and UNMIX.

Source apportionment of fine particulate matter (PM2.5, i.e., particles with an aerodynamic diameter of 2.5 microm or less) in Beijing, China, was determined using two eigenvector models, principal component analysis/absolute principal component scores (PCA/APCS) and UNMIX. The data used in this study were from the chemical analysis of 24-h samples, which were collected at 6-day intervals in January, April, July, and October 2000 in the Beijing metropolitan area. Both models identified five sources of PM2.5: secondary sulfate and secondary nitrate, a mixed source of coal combustion and biomass burning, industrial emission, motor vehicles exhaust, and road dust. On average, the PCA/APCS and UNMIX models resolved 73% and 85% of the PM2.5 mass concentrations, respectively. The results were comparable to previous estimate using the positive matrix factorization (PMF) and chemical mass balance (CMB) receptor models. Secondary products and the emissions from coal combustion and biomass burning dominated PM2.5. Such comparison among various receptor models, which contain different physical constraints, is important for better understanding PM2.5 sources.

Air Pollutants↗

Characteristics of PM10, SO2, NO(x) and O3 in ambient air during the dust storm period in Beijing.

In this study, the hourly variations of the mass concentrations of PM10, SO2, NO(x) and O3 at three sampling sites were observed in Beijing during dust storm occurrence period in April 2000. The PM2.5 samples were simultaneously collected. By comparing the hourly variations of the pollutant concentrations before, during and after dust storm event and haze pollution episode, the variation characteristics of the mass concentrations of PM10, SO2, NO(x) and O3 during dust storm events were presented. The results show that the mass concentration of PM10 reached 1500 microg m(-3) during dust storm events on April 6 and 25, 2000, which was 5-10 times that of the non-dust weather conditions, and this period of high mass concentration of PM10 lasted for about 14 h, and then the concentration level prior to the dust event was recovered in 6-h time period. Due to the strong wind, the concentrations of SO2, NO(x), NO2 and O3 during dust storm period were maintained at low levels, which was significantly different from those on non-dust storm and haze pollution conditions. A lot of coarse particles as well as a very large amount of fine particles were contained in the atmospheric particulates during dust storm period, and the concentration level of PM2.5 was comparable to that during haze pollution episode. During the dust storm period, the PM2.5 concentration was approximately 230 microg m(-3), accounting for 30% of the total PM10 mass concentration, was four times that of non-dust weather conditions, and the crustal elements constituted about 66.4% of the chemical composition of PM2.5 while sulfate and nitrate contributed much less, which was quite different from the chemical composition of PM2.5 primarily constituted by sulfate, nitrate and organics on haze pollution day.

Air↗

[Source apportionment on fine particles in Beijing].

The positive matrix factorization(PMF) method was used to apportion the sources for fine particles in Beijing. The data were obtained from four samplings from 1999 to 2000. The number of this data set was 40. The chemical compositions used in analysis include element carbon(EC), organics, SO4(2-), F-, Cl-, Fe, Ca, K, Mg, Al, Na, Zn, Mn, Ti, Pb, Ba and P. Six main sources, soil dust, construction dust, secondary source (by photochemical action), biomass burning, motor vehicle and coal burning were found.

Air Pollutants↗