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M R Tarbutt

Publications and source records attributed to M R Tarbutt.

3 recordsLinked to original sources

Stark shift of the A2Pi(1/2) state in 174YbF.

We have measured the Stark shift of the A2Pi(1/2)-X2Sigma+ transition in YbF. We use a molecular beam triple resonance method, with two laser transitions acting as pump and probe, assisted by an rf transition that tags a single hyperfine transition of the X state. After subtracting the known ground state Stark shift, we obtain a value of 70.3(1.5) Hz/(V/cm)2 for the static electric polarizability of the state A2Pi(1/2) (J=1/2),f by fitting our data to a purely quadratic Stark shift in the interval 0-5 kV/cm. A more exact analysis that does not assume a perfectly quadratic Stark effect yields the value mu(e)=2.48(3) D for the electric dipole moment of the A2Pi(1/2)(v=0) state.

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Slowing heavy, ground-state molecules using an alternating gradient decelerator.

We have decelerated a supersonic beam of 174YbF molecules using a switched sequence of electrostatic field gradients. These molecules are 7 times heavier than any previously decelerated. An alternating gradient structure allows us to decelerate and focus the molecules in their ground state. We show that the decelerator exhibits the axial and transverse stability required to bring the molecules to rest. Our work significantly extends the range of molecules amenable to this powerful method of cooling and trapping.

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Measurement of the electron electric dipole moment using YbF molecules.

The most sensitive measurements of the electron electric dipole moment d(e) have previously been made using heavy atoms. Heavy polar molecules offer a greater sensitivity to d(e) because the interaction energy to be measured is typically 10(3) times larger than in a heavy atom. We have used YbF to make the first measurement of this kind. Together, the large interaction energy and the strong tensor polarizability of the molecule make our experiment essentially free of the systematic errors that currently limit d(e) measurements in atoms. Our first result d(e) = (-0.2+/-3.2)x10(-26)e cm is less sensitive than the best atom measurement but is limited only by counting statistics and demonstrates the power of the method.

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