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Michael F Schatz

Publications and source records attributed to Michael F Schatz.

5 recordsLinked to original sources

Chaotic mixing in microdroplets.

We describe a general methodology for introducing thorough chaotic mixing in microdroplets. The mixing properties of fluid flows in microdroplets are governed by their symmetries, which give rise to invariant surfaces serving as barriers to transport. Complete three-dimensional mixing by chaotic advection requires destruction of all flow invariants. To illustrate this idea, we demonstrate that complete mixing can be obtained in a time-dependent flow produced by moving a microdroplet along a two-dimensional path. The theoretical predictions are confirmed by experiments that use the thermocapillary effect to manipulate microdroplets.

Diffusion↗

Complex-ordered patterns in shaken convection.

We report and analyze complex patterns observed in a combination of two standard pattern forming experiments. These exotic states are composed of two distinct spatial scales, each displaying a different temporal dependence. The system is a fluid layer experiencing forcing from both a vertical temperature difference and vertical time-periodic oscillations. Depending on the parameters these forcing mechanisms produce fluid motion with either a harmonic or a subharmonic temporal response. Over a parameter range where these mechanisms have comparable influence the spatial scales associated with both responses are found to coexist, resulting in complex, yet highly ordered patterns. Phase diagrams of this region are reported and criteria to define the patterns as quasiperiodic crystals or superlattices are presented. These complex patterns are found to satisfy four-mode (resonant tetrad) conditions. The qualitative difference between the present formation mechanism and the resonant triads ubiquitously used to explain complex-ordered patterns in other nonequilibrium systems is discussed. The only exception to quantitative agreement between our analysis based on Boussinesq equations and laboratory investigations is found to be the result of breaking spatial symmetry in a small parameter region near onset.

Journal Article↗

Secondary instabilities of hexagonal patterns in a Bénard-Marangoni convection experiment.

We have identified experimentally secondary instability mechanisms that restrict the stable band of wave numbers for ideal hexagons in Bénard-Marangoni convection. We use "thermal laser writing" to impose long wave perturbations of ideal hexagonal patterns as initial conditions and measure the growth rates of the perturbations. For epsilon=0.46 our results suggest a longitudinal phase instability limits stable hexagons at a high wave number while a transverse phase instability limits low wave number hexagons.

Journal Article↗

Optical manipulation of microscale fluid flow.

A novel optical method is used both to probe and to control dynamics in experiments on the spreading of microscale liquid films over solid substrates. The flow is manipulated by thermally induced surface-tension gradients that are regulated by controlling the absorption of light in the substrate. This approach permits, for the first time, the measurement of the dispersion relation for the well-known contact line instability; the measurements are compared with theoretical predictions from the slip model for spreading films. The experiments also demonstrate the use of feedback control to suppress instability. These results show that optical control can provide dynamically reconfigurable manipulations of fluid flow, thereby suggesting a general approach for constructing reprogrammable microfluidic devices.

Journal Article↗

Evolution of hexagonal patterns from controlled initial conditions in a Bénard-Marangoni convection experiment.

We report quantitative measurements of both wave number selection and defect motion in nonequilibrium hexagonal patterns. A novel optical technique ("thermal laser writing") is used to imprint initial patterns with selected characteristics in a Bénard-Marangoni convection experiment. Initial patterns of ideal hexagons are imposed to determine the band of stable pattern wave numbers while initial patterns containing an isolated penta-hepta defect are imprinted to study defect propagation directions and velocities. The experimental results are compared to recent theoretical predictions.

Journal Article↗