Biomedical subjects

Michael Twardos

Publications and source records attributed to Michael Twardos.

5 recordsLinked to original sources

PubMed2006

Characterization of anomalous flow and phase behavior in a Langmuir monolayer of 2-hydroxy-tetracosanoic acid.

Langmuir monolayers of long-chain fatty acids display a wide range of interesting flow and phase behaviors, but the correlation between these behaviors varies. In this paper, we report two interesting behaviors in a Langmuir monolayer of 2-hydroxy-tetracosanoic acid: phase coexistence between the L(2h) and L(2)' phases over a large pressure range and a peak in the viscosity and elastic modulus of the material as a function of pressure. The two behaviors are confirmed over a range of temperatures for which the location of the undistorted lattice appears to vary relative to the range of coexistence for the two phases. Evidence for a correlation between the phase behavior and the peak in the mechanical properties is presented.

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PubMed2006

Asymmetric response of a jammed plastic bead raft.

The successful development of an effective temperature would be an important step in the application of statistical mechanics principles to systems driven far from equilibrium. One direction that has shown promise is the use of fluctuation-dissipation relations. However, driven systems break time-reversal symmetry, and understanding the implications of this for fluctuation-dissipation relations is a critical step in developing effective temperatures. Here we study the response function in a driven system of plastic beads as a function of the density in order to elucidate the generality of the use of fluctuation-dissipation relations. We find that even when a linear response is observed, the time scale of the response is dependent on the direction of the applied stress.

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PubMed2005

Comparison between step strains and slow steady shear in a bubble raft.

We report on a comparison between stress relaxations after an applied step strain and stress relaxations during slow, continuous strain in a bubble raft. A bubble raft serves as a model two-dimensional foam and consists of a single layer of bubbles on a water surface. For both step strains and continuous strain, one observes periods of stress increase and decrease. Our focus is on the distribution of stress decreases, or stress drops. The work is motivated by apparent disagreements between quasistatic simulations of flowing foam and simulations of continuous strain for foam. Quasistatic simulations have reported larger average stress drops than the continuous strain case. Also, there is evidence in quasistatic simulations for a general divergence of the average size of the stress drops that only appears to occur in steady strain near special values of the foam density. In this work, applied step strains are used as an approximation to quasistatic simulations. We find general agreement in the dependence of the average stress drop on rate of strain, but we do not observe evidence for a divergence of the average stress drop.

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PubMed2002

Folding Langmuir monolayers.

The maximum pressure a two-dimensional surfactant monolayer is able to withstand is limited by the collapse instability towards formation of three-dimensional material. We propose a new description for reversible collapse based on a mathematical analogy between the formation of folds in surfactant monolayers and the formation of Griffith Cracks in solid plates under stress. The description, which is tested in a combined microscopy and rheology study of the collapse of a single-phase Langmuir monolayer (LM) of 2-hydroxy-tetracosanoic acid (2-OH TCA), provides a connection between the in-plane rheology of LMs and reversible folding.

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PubMed2002

Shear-induced stress relaxation in a two-dimensional wet foam.

We report on experimental measurements of the flow behavior of a wet, two-dimensional foam under conditions of slow, steady shear. The initial response of the foam is elastic. Above the yield strain, the foam begins to flow. The flow consists of irregular intervals of elastic stretch followed by sudden reductions of the stress, i.e., stress drops. We report on the distribution of the stress drops as a function of the applied shear rate. We also comment on our results in the context of various two-dimensional models of foams.

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