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N Bernhoeft

Publications and source records attributed to N Bernhoeft.

5 recordsLinked to original sources

63Cu nuclear relaxation in the quantum critical point system CeCu5.9Au0.1.

63Cu NQR measurements of the 63Cu T1 are reported for the quantum critical point system CeCu5.9Au0.1 over temperatures ranging from 0.1 up to 4.2 K. Below approximately 1 K the magnetization recovery exhibits a stable, nonexponential decay function which we believe signals the onset of 2D quantum critical fluctuations, as has been noted in the literature. We find T1(-1) is proportional to T0.75 for the region T < 1 K. The observed temperature dependence is in agreement with a phenomenological model of non-Fermi liquid behavior based on the uniform susceptibility but is inconsistent with calculations based on susceptibility peaks identified via neutron scattering experiments.

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Magnetic ground state of pure and doped CeFe2.

A combination of neutron elastic and inelastic, resonant x-ray scattering, and 57Fe Mössbauer experiments are used to determine the unusual magnetic ground state of CeFe2. The complementarities between different time-scale techniques may allow one to understand the dynamic features of the ground state in CeFe2 and its pseudobinary compounds, and how the frustration of Fe tetrahedra leads the appearance of antiferromagnetic fluctuations in the presence of ferrimagnetism. The resulting model can be used to rationalize many of the unusual and conflicting experimental results reported for this material in the literature.

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Triple-q(-->) octupolar ordering in NpO2.

We report the results of resonant x-ray scattering experiments performed at the Np M(4,5) edges in NpO2. Below T(0)=25 K, the development of long-range order of Np electric quadrupoles is revealed by the growth of superlattice Bragg peaks. The polarization and azimuthal dependence of the intensity of the resonant peaks are well reproduced assuming anisotropic tensor susceptibility scattering from a triple-q(-->) longitudinal antiferroquadrupolar structure. Electric-quadrupole order in NpO2 could be driven by the ordering at T0 of magnetic octupoles of Gamma(5) symmetry, splitting the Np ground state quartet and leading to a singlet ground state with zero dipole-magnetic moment.

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Resonant enhancements at nonmagnetic ions: new possibilities for magnetic X-ray scattering.

Synchrotron experiments with uranium antiferromagnetic compounds have discovered large ( >1000) enhancements of the magnetic scattering intensities at the K edges of nominally nonmagnetic anions, e.g., Ga and As. The width in energy, the position with respect to the white line, and the azimuthal and polarization dependencies permit one to associate the signal with transitions of E1 dipole symmetry from 1s to 4p states. In momentum space, the signal exhibits long-range order at the antiferromagnetic wave vector. We discuss possible channels capable of generating the observed enhancements.

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Geometrical effects in diffraction analysis.

The use of X-ray and neutron scattering as a tool to study phase transitions is well established. As techniques improve and experiments are made under successively higher resolution, the need to consider the role of both the distribution of diffracting length scales and the incident-beam coherence volume is emphasized. The interplay of diffracting length scales and the beam coherence volume no longer permits calculation of diffraction profiles in terms of the sample intensity response convolved with an instrumental resolution function. Rather, the probe and sample now enter the calculation on an equal footing at the level of the scattering amplitudes. Under these conditions, it is found that the summation of coherent scattering amplitudes leads to characteristic profiles in wave-vector and, in the case of resonant X-ray scattering, energy space. In this latter case, in the vicinity of strong absorption edges, as used for example in resonant magnetic X-ray diffraction, the energy dependence of diffraction profiles may uniquely allow spatial localization of the scattering volume below the sample surface. This observation may considerably augment the range and power of resonant X-ray scattering.

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