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P B Littlewood

Publications and source records attributed to P B Littlewood.

16 recordsLinked to original sources

Bose-Einstein condensation of exciton polaritons.

Phase transitions to quantum condensed phases--such as Bose-Einstein condensation (BEC), superfluidity, and superconductivity--have long fascinated scientists, as they bring pure quantum effects to a macroscopic scale. BEC has, for example, famously been demonstrated in dilute atom gas of rubidium atoms at temperatures below 200 nanokelvin. Much effort has been devoted to finding a solid-state system in which BEC can take place. Promising candidate systems are semiconductor microcavities, in which photons are confined and strongly coupled to electronic excitations, leading to the creation of exciton polaritons. These bosonic quasi-particles are 10(9) times lighter than rubidium atoms, thus theoretically permitting BEC to occur at standard cryogenic temperatures. Here we detail a comprehensive set of experiments giving compelling evidence for BEC of polaritons. Above a critical density, we observe massive occupation of the ground state developing from a polariton gas at thermal equilibrium at 19 K, an increase of temporal coherence, and the build-up of long-range spatial coherence and linear polarization, all of which indicate the spontaneous onset of a macroscopic quantum phase.

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Nonequilibrium quantum condensation in an incoherently pumped dissipative system.

We study spontaneous quantum coherence in an out of an equilibrium system, coupled to multiple baths describing pumping and decay. For a range of parameters describing coupling to, and occupation of the baths, a stable steady-state condensed solution exists. The presence of pumping and decay significantly modifies the spectra of phase fluctuations, leading to correlation functions that differ both from an isolated condensate and from a laser.

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Thermodynamics and excitations of condensed polaritons in disordered microcavities.

We study the thermodynamic condensation of microcavity polaritons using a realistic model of disorder in semiconductor quantum wells. This approach correctly describes the polariton inhomogeneous broadening in the low density limit, and treats scattering by disorder to all orders in the condensed regime. While the weak disorder changes the thermodynamic properties of the transition little, the effects of disorder in the condensed state are prominent in the excitations and can be seen in resonant Rayleigh scattering.

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Solitonic phase in manganites.

Orbital order present in several transition metal compounds could give rise to topological defects. Here we argue that the topological defects in orbital ordered half doped manganites are orbital solitons that carry a charge of +/-e/2. When extra charge is added to the system an array of solitons is formed and an incommensurate solitonic phase occurs. The striking experimental asymmetry in the phase diagram as electrons or holes are added to half doped manganites is explained by the energy difference between positive and negative charged solitons. The presence of nanoscale inhomogeneities in manganites is naturally explained by the existence of solitonic phases.

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Weak charge-lattice coupling requires reinterpretation of stripes of charge order in La1-xCaxMnO3.

Modulations in manganites attributed to stripes of charge/orbital/spin order are thought to result from strong electron-lattice interactions that lock the superlattice and parent lattice periodicities. Surprisingly in La1-xCaxMnO3 (x>0.5,90 K), convergent beam (3.6 nm spot) electron diffraction patterns rule out charge stacking faults and indicate a superlattice with uniform periodicity. Moreover, large area electron diffraction peaks are sharper than simulations with stacking faults. Since the electron-lattice coupling does not lock the two periodicities (to yield stripes) it may be too weak to strongly localize charge.

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Electronically soft phases in manganites.

The phenomenon of colossal magnetoresistance in manganites is generally agreed to be a result of competition between crystal phases with different electronic, magnetic and structural order; a competition which can be strong enough to cause phase separation between metallic ferromagnetic and insulating charge-modulated states. Nevertheless, closer inspection of phase diagrams in many manganites reveals complex phases where the two order parameters of magnetism and charge modulation unexpectedly coexist. Here we show that such experiments can be naturally explained within a phenomenological Ginzburg-Landau theory. In contrast to models where phase separation originates from disorder or as a strain-induced kinetic phenomenon, we argue that magnetic and charge modulation coexist in new thermodynamic phases. This leads to a rich diagram of equilibrium phases, qualitatively similar to those seen experimentally. The success of this model argues for a fundamental reinterpretation of the nature of charge modulation in these materials, from a localized to a more extended 'charge-density wave' picture. The same symmetry considerations that favour textured coexistence of charge and magnetic order may apply to many electronic systems with competing phases. The resulting 'electronically soft' phases of matter with incommensurate, inhomogeneous and mixed order may be general phenomena in correlated systems.

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Polariton condensation with localized excitons and propagating photons.

We estimate the condensation temperature for microcavity polaritons, allowing for their internal structure. We consider polaritons formed from localized excitons in a planar microcavity, using a generalized Dicke model. At low densities, we find a condensation temperature T(c) proportional, rho, as expected for a gas of structureless polaritons. However, as T(c) becomes of the order of the Rabi splitting, the structure of the polaritons becomes relevant, and the condensation temperature is that of a BCS-like mean-field theory. We also calculate the excitation spectrum, which is related to observable quantities such as the luminescence and absorption spectra.

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Angular distribution of photoluminescence as a probe of bose condensation of trapped excitons.

Recent experiments on two-dimensional exciton systems have shown that excitons collect in shallow in-plane traps. We find that Bose condensation in a trap results in a dramatic change of the exciton photoluminescence (PL) angular distribution. The long-range coherence of the condensed state gives rise to a sharply focused peak of radiation in the direction normal to the plane. By comparing the PL profile with and without Bose condensation, we provide a simple diagnostic for the existence of a Bose condensate. The PL peak has strong temperature dependence due to the thermal order parameter phase fluctuations across the system. The angular PL distribution can also be used for imaging vortices in the trapped condensate. Vortex phase spatial variation leads to destructive interference of PL radiation in certain directions, creating nodes in the PL distribution that imprint the vortex configuration.

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Oxygen stripes in La0.5Ca0.5MnO3 from ab initio calculations.

We investigate the electronic, magnetic, and orbital properties of La0.5Ca0.5MnO3 perovskite by means of an ab initio electronic structure calculation within the Hartree-Fock approximation. Using the experimental crystal structure reported by Radaelli et al. [Phys. Rev. B 55, 3015 (1997)]], we find a charge-ordering stripelike ground state. The periodicity of the stripes, and the insulating magnetic structure, consisting of antiferromagnetically coupled zigzag chains, are in agreement with neutron x-ray and electron diffraction experiments. However, the detailed structure is more complex than that envisaged by simple models of charge and orbital order on Mn d levels alone, and is better described as a charge-density wave of oxygen holes, coupled to the Mn spin/orbital order.

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Non-saturating magnetoresistance in heavily disordered semiconductors.

The resistance of a homogeneous semiconductor increases quadratically with magnetic field at low fields and, except in very special cases, saturates at fields much larger than the inverse of the carrier mobility, a number typically of the order of 1 T (refs 1, 2). A surprising exception to this behaviour has recently been observed in doped silver chalcogenides, which exhibit an anomalously large, quasi-linear magnetoresistive response that extends down to low fields and survives, even at extreme fields of 55 T and beyond. Here we present a simple model of a macroscopically disordered and strongly inhomogeneous semiconductor that exhibits a similar non-saturating magnetoresistance. In addition to providing a possible explanation for the behaviour of doped silver chalcogenides, our model suggests potential routes for the construction of magnetic field sensors with a large, controllable and linear response.

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Collective density-wave excitations in two-leg Sr14-xCaxCu24O41 ladders.

Raman measurements in the 1.5-20 cm(-1) energy range were performed on single crystals of Sr14-xCaxCu24O41. A quasielastic scattering peak (QEP) which softens with cooling is observed only in the polarization parallel to the ladder direction for samples with x=0, 8, and 12. The QEP is a Raman fingerprint of pinned collective density wave excitations screened by uncondensed carriers in the ladder structures. Our results suggest that transport in metallic samples, which is similar to transport in underdoped high-T(c) cuprates, is driven by a collective electronic response.

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Schrödinger equation with a spatially and temporally random potential: effects of cross-phase modulation in optical communication.

We model the effects of cross-phase modulation in frequency (or wavelength) division multiplexed optical communications systems, using a Schrödinger equation with a spatially and temporally random potential. Green's functions for the propagation of light in this system are calculated using Feynman path-integral and diagrammatic techniques. This propagation leads to a non-Gaussian joint distribution of the input and output optical fields. We use these results to determine the amplitude and timing jitter of a signal pulse and to estimate the system capacity in analog communication.

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Acoustically induced stark effect for excitons in intrinsic semiconductors.

A Stark effect for excitons parametrically driven by coherent acoustic phonons is proposed. Our scheme refers to a low-temperature intrinsic semiconductor or semiconductor nanostructure pumped by an acoustic wave (frequency band nu(ac) approximately equal to 1-40 GHz and intensity range I(ac) approximately equal to 10(-2)-10(2) W/cm(2)) and probed by low-intensity light. Tunable optical band gaps, which strongly change the spectral shape of the exciton line, are induced in the polariton spectrum by acoustic pumping. We develop an exactly solvable model of the acoustic Stark effect and apply our results to GaAs driven by bulk or surface acoustic waves.

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Stimulated scattering of indirect excitons in coupled quantum wells: signature of a degenerate Bose-gas of excitons.

We observe and analyze strongly nonlinear photoluminescence kinetics of indirect excitons in GaAs/AlGaAs coupled quantum wells at low bath temperatures, > or = 50 mK. The long recombination lifetime of indirect excitons promotes accumulation of these Bose particles in the lowest energy states and allows the photoexcited excitons to cool down to temperatures where the dilute 2D gas of indirect excitons becomes statistically degenerate. Our main result--a strong enhancement of the exciton scattering rate to the low-energy states with increasing concentration of the indirect excitons--reveals bosonic stimulation of exciton scattering, which is a signature of a degenerate Bose-gas of excitons.

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Coexistence of superconductivity and ferromagnetism in ferromagnetic metals.

We address the question of coexistence of superconductivity and ferromagnetism. Using a field theoretical approach we study a one-fermion effective model of a ferromagnetic superconductor in which the quasiparticles responsible for the ferromagnetism form the Cooper pairs as well. For the first time we solve self-consistently the mean-field equations for the superconducting gap and the spontaneous magnetization. We discuss the physical features which are different in this model and the standard BCS model and consider their experimental consequences.

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