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P G Lagoudakis

Publications and source records attributed to P G Lagoudakis.

3 recordsLinked to original sources

Wave function engineering in elongated semiconductor nanocrystals with heterogeneous carrier confinement.

We explore two routes to wave function engineering in elongated colloidal CdSe/CdS quantum dots, providing deep insight into the intrinsic physics of these low-dimensional heterostructures. Varying the aspect ratio of the nanoparticle allows control over the electron-hole overlap (radiative rate), and external electric fields manipulate the interaction between the delocalized electron and the localized hole. In agreement with theory, this leads to an exceptional size dependent quantum confined Stark effect with field induced intensity modulations, opening applications as electrically switchable single photon sources.

Journal Article↗

Experimental evidence for exciton scaling effects in self-assembled molecular wires.

Resonant Rayleigh scattering from self-assembled one-dimensional molecular J-aggregate wires reveals a distinct dependence of the exciton energy on the width of lateral extension. For the J aggregates used in this study, strong in-line dipole coupling leads to a delocalization of the exciton wave function over several molecular units. Polarization dependent measurements of resonantly scattered light from the wires show that the exciton dipole moment is oriented perpendicular to the long axis. The experimental observations can be described by applying a quantization condition to the center of mass motion of the J-band exciton in the wires.

Journal Article↗

Electron-polariton scattering in semiconductor microcavities.

In semiconductor microcavities, electron-polariton scattering has been proposed as an efficient process that can drive polaritons from the bottleneck region to the ground state, achieving Bose amplification of the optical emission. We present clear experimental observation of this process in a structure that allows control of the electron density and we report substantial enhancement of photoluminescence. We show that this enhancement is more effective at higher temperatures due to the different way that electron scattering processes either broaden or relax polaritons.

Journal Article↗