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P Hawrylak

Publications and source records attributed to P Hawrylak.

At least 19 recordsLinked to original sources

Stability diagram of a few-electron triple dot.

Individual and coupled quantum dots containing one or two electrons have been realized and are regarded as components for future quantum information circuits. In this Letter we map out experimentally the stability diagram of the few-electron triple dot system, the electron configuration map as a function of the external tuning parameters, and reveal experimentally for the first time the existence of quadruple points, a signature of the three dots being in resonance. In the vicinity of these quadruple points we observe a duplication of charge transfer transitions related to charge and spin reconfigurations triggered by changes in the total electron occupation number. The experimental results are largely reproduced by equivalent circuit analysis and Hubbard models. Our results are relevant for future quantum mechanical engineering applications within both quantum information and quantum cellular automata architectures.

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Remanent zero field spin splitting of self-assembled quantum dots in a paramagnetic host.

We report on the observation of a finite spin splitting at zero magnetic field in resonant tunneling experiments on CdSe self-assembled quantum dots in a (Zn,Be,Mn)Se barrier. This is remarkable since bulk II-VI dilute magnetic semiconductors are paramagnets. Our experiment may be viewed as tunneling through a single magnetic polaron, where the carriers contained inside the dot act to mediate an effective ferromagnetic interaction between Mn ions in their vicinity. The effect is observable up to relatively high temperatures, which we tentatively ascribe to a feedback mechanism with the electrical current, previously predicted theoretically.

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Excitonic energy shell structure of self-assembled InGaAs/GaAs quantum dots.

Performing optical spectroscopy of highly homogeneous quantum dot arrays in ultrahigh magnetic fields, an unprecedently well resolved Fock-Darwin spectrum is observed. The existence of up to four degenerate electronic shells is demonstrated where the magnetic field lifts the initial degeneracies, which reappear when levels with different angular momenta come into resonance. The resulting level shifting and crossing pattern also show evidence of many-body effects such as the mixing of configurations and exciton condensation at the resonances.

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Exciton dephasing in quantum dot molecules.

We have measured the exciton dephasing time in InAs/GaAs quantum dot molecules having different interdot barrier thicknesses in the temperature range from 5 to 60 K, using a highly sensitive four-wave mixing heterodyne technique. At 5 K dephasing times of several hundred picoseconds are found. Moreover, a systematic dependence of the dephasing dynamics on the barrier thickness is observed. These results show how the quantum-mechanical coupling of the electronic wave functions in the molecules affects both the exciton radiative lifetime and the exciton-acoustic phonon interaction.

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Spin-blockade spectroscopy of a two-level artificial molecule.

Coulomb- and spin-blockade spectroscopy investigations have been performed on an electrostatically defined "artificial molecule" connected to spin polarized leads. The molecule is first effectively reduced to a two-level system by placing both constituent atoms at a specific location of the level spectrum. The spin sensitivity of the conductance enables us to identify the electronic spin states of the two-level molecule. We find in addition that the magnetic field induces variations in the tunnel coupling between the two atoms. The lateral nature of the device is evoked to explain this behavior.

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Optical detection of the Aharonov-Bohm effect on a charged particle in a nanoscale quantum ring.

We study spectroscopically the current produced by a charged particle moving in a nanosize semiconductor quantum ring subject to a perpendicular magnetic field. Several Aharonov-Bohm oscillations are observed in the emission of a charged exciton confined in a single ring structure. The magnetic field period of the oscillations correlates well with the size of the rings.

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Fine structure of excitons in InAs/GaAs coupled auantum dots: a sensitive test of electronic coupling.

Exciton fine structure in InAs/GaAs coupled quantum dots has been studied by photoluminescence spectroscopy in magnetic fields up to 8 T. Pronounced anticrossings and mixings of optically bright and dark states as functions of magnetic field are seen. A theoretical treatment of the mixing of the excitonic states has been developed, and it traces observed features to structural asymmetries. These results provide direct evidence for coherent coupling of excitons in quantum dot molecules.

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Collapse of the spin-singlet phase in quantum dots.

We present experimental and theoretical results on a new regime in quantum dots in which the filling factor two-singlet state is replaced by new spin polarized phases. We make use of spin blockade spectroscopy to identify the transition to this new regime as a function of the number of electrons. The key experimental observation is a reversal of the phase in the systematic oscillation of the amplitude of Coulomb blockade peaks as the number of electrons is increased above a critical number. It is found theoretically that correlations are crucial to the existence of the new phases.

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Coupling and entangling of quantum states in quantum dot molecules.

We demonstrate coupling and entangling of quantum states in a pair of vertically aligned, self-assembled quantum dots by studying the emission of an interacting electron-hole pair (exciton) in a single dot molecule as a function of the separation between the dots. An interaction-induced energy splitting of the exciton is observed that exceeds 30 millielectron volts for a dot layer separation of 4 nanometers. The results are interpreted by mapping the tunneling of a particle in a double dot to the problem of a single spin. The electron-hole complex is shown to be equivalent to entangled states of two interacting spins.

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Excitonic absorption in a quantum Dot

The excitonic absorption spectrum of a single quantum dot is investigated theoretically and experimentally. The spectrum is determined by an interacting electron-valence-hole complex. We show that the mixing of quantum configurations by two-body interactions leads to distinct absorption spectra controlled by the number of confined electronic shells. The theoretical results are compared with results of photoluminescence excitation spectroscopy on a series of single self-assembled In0.60Ga0.40As quantum dots.

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Hidden symmetries in the energy levels of excitonic 'artificial atoms'

Quantum dots or 'artificial atoms' are of fundamental and technological interest--for example, quantum dots may form the basis of new generations of lasers. The emission in quantum-dot lasers originates from the recombination of excitonic complexes, so it is important to understand the dot's internal electronic structure (and of fundamental interest to compare this to real atomic structure). Here we investigate artificial electronic structure by injecting optically a controlled number of electrons and holes into an isolated single quantum dot. The charge carriers form complexes that are artificial analogues of hydrogen, helium, lithium, beryllium, boron and carbon excitonic atoms. We observe that electrons and holes occupy the confined electronic shells in characteristic numbers according to the Pauli exclusion principle. In each degenerate shell, collective condensation of the electrons and holes into coherent many-exciton ground states takes place; this phenomenon results from hidden symmetries (the analogue of Hund's rules for real atoms) in the energy function that describes the multi-particle system. Breaking of the hidden symmetries leads to unusual quantum interferences in emission involving excited states.

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