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P Lambropoulos

Publications and source records attributed to P Lambropoulos.

At least 19 recordsLinked to original sources

Ab initio investigation of the phase lag in coherent control of H(2).

An ab initio investigation of the excitation of an H(2) resonance, coupled to ionization and dissociation continua, was performed. The excitation occurs via a one- and a three-photon path where both fields have a variable but well-defined phase relation. While both continuum yields show an oscillatory behavior as the phase is varied, a pronounced phase lag between the two oscillations is observed, if the excitation energy is detuned from the resonant transition. The results are discussed in connection to a recent series of experiments performed on HI and the subsequent discussion on the possible origin of the observed phase lag.

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Phase control of photoabsorption in optically dense media

We present a self-consistent theory, as well as an illustrative application to a realistic system, of phase control of photoabsorption in an optically dense medium. We demonstrate that, when propagation effects are taken into consideration, the impact on phase control is significant. Independent of the value of the initial phase difference between the two fields, over a short scaled distance of propagation, the medium tends to settle the relative phase so that it cancels the atomic excitation. In addition, we find some rather unusual behavior for an optically thin layer.

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Laser-induced transitions between triply excited hollow states

We present an ab initio calculation of the Li+ photoion yield in the presence of laser coupling between the triply excited 2s(2)2p(2)P(o) and 2s2p(2) (2)D(e) resonances in lithium, the first of which is assumed excited by synchrotron radiation from the ground state. The laser coupling between the triply excited states is shown to lead to a significant and readily measurable modification of the line profile which provides a unique probe of the dipole strength between highly correlated triply excited states.

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