Biomedical subjects

P Monceau

Publications and source records attributed to P Monceau.

At least 19 recordsLinked to original sources

PubMed2006

Subgap collective tunneling and its staircase structure in charge density waves.

Tunneling spectra of chain materials NbSe3 and TaS3 were studied in nanoscale mesa devices. Current-voltage I-V characteristics related to all charge density waves (CDWs) reveal universal spectra within the normally forbidden region of low V, below the electronic CDW gap 2Delta. The tunneling always demonstrates a threshold Vt approximately 0.2Delta, followed, for both CDWs in NbSe3, by a staircase fine structure. T dependencies of Vt(T) and Delta(T) scale together for each CDW, while the low T values Vt(0) correlate with the CDWs' transition temperatures Tp. Fine structures of CDWs perfectly coincide when scaled along V/Delta. The results evidence the sequential entering of CDW vortices (dislocations) in the junction area with the tunneling current concentrated in their cores. The subgap tunneling proceeds via the phase channel: coherent phase slips at neighboring chains.

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PubMed2005

Observation of charge density wave solitons in overlapping tunnel junctions.

We report on direct observation of microscopic solitons in single electronic processes of the coherent interlayer tunneling in charge density waves. Special nanoscale devices were fabricated from the chain compound using focused ion beams. The spectra were drastically refined by working at high (up to 27 T) magnetic fields. Internal quantum tunneling of electrons can go through solitons that are energetically more favorable quantum particles than electrons. In addition to the interband tunneling across the gap 2Delta, we observe a clear peak at the intermediate voltage approximately 2Delta/3, which we associate with the creation of microscopic solitons, the energy of which must be 2Delta/pi. These solitons might correspond to the long sought special quasiparticle--the spinon.

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PubMed2004

Sliding-induced decoupling and charge transfer between the coexisting Q1 and Q2 charge density waves in NbSe3.

Using high-resolution x-ray scattering in the presence of an applied current, we report evidence for a dynamical decoupling between the two NbSe3 charge-density waves (CDWs), Q1 (T(C1)=145 K) and Q2 (T(C2)=59 K), coexisting below T(C2). Simultaneous and oppositely directed shifts of the relevant CDW superlattice spots develop above a threshold current which we identify as the depinning threshold I(C1) for the more strongly pinned upper CDW Q1 (I(C1) approximately 10I(C2)). In contrast with shifts induced by current conversion processes, the present effect is not current polarized and is not limited to the current-contact regions. We propose a model which explains this instability through a sliding-induced charge transfer between the two electronic reservoirs corresponding to the Q1 and Q2 CDWs.

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PubMed2003

Evidence of 1D behavior of He4 confined within carbon-nanotube bundles.

We present the first low-temperature thermodynamic investigation of the controlled physisorption of He4 gas in carbon single-wall nanotube (SWNT) samples. The vibrational specific heat measured between 100 mK and 6 K demonstrates an extreme sensitivity to outgassing conditions. For bundles with a few number of nanotubes the extra contribution to the specific heat, C(ads), originating from adsorbed He4 at very low density displays 1D behavior, typical for He atoms localized within linear channels as grooves and interstitials, for the first time evidenced. For larger bundles, C(ads) recovers the 2D behavior akin to the case of He4 films on planar substrates (grafoil).

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PubMed2002

Motional ordering of a charge-density wave in the sliding state.

We have used high-resolution x-ray scattering, in the presence of an applied direct current, for studying the correlation lengths in the sliding charge-density wave (CDW) state. Transport properties were simultaneously measured in situ during the experiment. We find that, while the transverse correlation is reduced when the CDW moves, the CDW becomes more ordered in the direction of motion. This is the first report of a motional ordering process in a periodic system other than a vortex lattice.

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PubMed2001

Structural evidence for Ta-tetramerization displacements in the charge-density-wave compound (TaSe4)2I from x-ray anomalous diffraction.

We use the anomalous x-ray diffraction technique to investigate the nature of the tantalum displacement pattern in the modulated phase of the charge-density-wave compound (TaSe4)2I. In addition to the known acousticlike modulation, we find the first direct evidence for the condensation of opticlike Ta displacements along the metallic chains corresponding to an LLSS pattern of long and short in-chain Ta-Ta distances (Ta-tetramerization modes). This result confirms a previous model in which the interaction of the electronically coupled optic modes with long-wavelength acoustic shear modes leads to the condensation of a modulation of mixed character.

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PubMed2001

Ferroelectric Mott-Hubbard phase of organic (TMTTF)2X conductors.

We present experimental evidence and a corresponding theory for the ferroelectric transition in the family of quasi-one-dimensional conductors (TMTTF)2X. We interpret this new transition in the frame of the combined Mott-Hubbard state taking into account the double action of the spontaneous charge disproportionation on the TMTTF molecular stacks and of the X anionic potentials.

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PubMed2000

Convective terms and transversely driven charge-density waves

We derive the convective terms in the damping which determine the structure of the moving charge-density wave (CDW), and study the effect of a current flowing transverse to conducting chains on the CDW dynamics along the chains. In contrast to a recent prediction we find that the effect is orders of magnitude smaller, and that contributions from transverse currents of electron- and holelike quasiparticles to the force exerted on the CDW along the chains act in the opposite directions. We discuss recent experimental verification of the effect and demonstrate experimentally that geometry effects might mimic the transverse current effect.

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PubMed2000

Charge-density-wave current conversion in submicron NbSe3 wires

We have studied the charge-density-wave (CDW) current conversion process in NbSe3 wire structures of mesoscopic dimensions. A significant reduction of the phase-slip voltage associated with this conversion is observed if the spacing between current contacts is smaller than a few &mgr;m. This reduction cannot be explained with existing models of CDW current conversion. We suggest that single phase-slip events play a central role in micron-sized systems. The removal and addition of wave fronts may then become correlated in time.

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PubMed1996