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Patrick C Chaumet

Publications and source records attributed to Patrick C Chaumet.

10 recordsLinked to original sources
PubMed2006

Local-field enhancement in an optical force metallic nanotrap: application to single-molecule spectroscopy.

We study the local-field enhancement in a nanocavity created by optical nanomanipulation. Recently we showed that a metallic probe can modify the optical force experienced by a metallic particle and generate a material selective trapping potential. We show that the same configuration used for optical forces can be used to control both in magnitude and tune the local-field enhancement around the particle at resonance. The spatial resolution and material selectivity of this technique, allied to its capability to manipulate particles at the nanometric level, may offer a new and versatile way to achieve surface-enhanced Raman scattering spectroscopy at the single-molecule level.

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PubMed2006

Coupled dipole method for radiation dynamics in finite photonic crystal structures.

We present a coupled-dipole treatment of radiation dynamics in the weak-coupling regime in a finite three-dimensional photonic crystal structure. The structure is discretized in real space and the self-consistent local field is computed. We illustrate the computation of radiation dynamics by calculating the spontaneous emission rate for a source located in a defect cavity inside a slab photonic crystal structure. We compute the cavity spectral response, the near-field modal structure, and the far-field radiation pattern of the microcavity. We also discuss our results in light of the recent experimental near-field observations of the optical modes of a photonic crystal microcavity.

Journal Article↗
PubMed2006

Influence of multiple scattering on three-dimensional imaging with optical diffraction tomography.

Optical diffraction tomography is an imaging technique that permits retrieval of the map of permittivity of an object from its scattered far field. Most reconstruction procedures assume that single scattering is dominant so that the scattered far field is linearly linked to the permittivity. In this work, we present a nonlinear inversion method and apply it to complex three-dimensional samples. We show that multiple scattering permits one to obtain a power of resolution beyond the classical limit imposed by the use of propagative incident and diffracted waves. Moreover, we stress that our imaging method is robust with respect to correlated and uncorrelated noise.

Journal Article↗
PubMed2006

Fully vectorial highly nonparaxial beam close to the waist.

I use the angular spectrum representation to compute exactly the Gaussian beam close to the waist (w(0)) in the case of a highly nonparaxial field (w(0)<lambda). The computation is done in the vectorial case for a polarized Gaussian beam. In the area of the waist, the contribution of the propagating and evanescent waves is discussed. Moreover, the Gaussian wave is developed in terms of a series, which permits one to get analytical expressions for both propagating and evanescent waves when the observation is close to the waist.

Journal Article↗
PubMed2005

Efficient computation of optical forces with the coupled dipole method.

We present computational techniques to compute in an efficient way optical forces on arbitrary nanoobjects using the coupled dipole method. We show how the time of computation can be reduced by several orders of magnitude with the help of fast-Fourier-transform techniques. We also discuss the influence of different formulations of the electric polarizability of a small scatterer on the accuracy and robustness of the computation of optical forces.

Journal Article↗
PubMed2005

Superresolution in total internal reflection tomography.

We simulate a total internal reflection tomography experiment in which an unknown object is illuminated by evanescent waves and the scattered field is detected along several directions. We propose a full-vectorial three-dimensional nonlinear inversion scheme to retrieve the map of the permittivity of the object from the scattered far-field data. We study the role of the solid angle of illumination, the incident polarization, and the position of the prism interface on the resolution of the images. We compare our algorithm with a linear inversion scheme based on the renormalized Born approximation and stress the importance of multiple scattering in this particular configuration. We analyze the sensitivity to noise and point out that using incident propagative waves together with evanescent waves improves the robustness of the reconstruction.

Journal Article↗
PubMed2004

Superresolution of three-dimensional optical imaging by use of evanescent waves.

We simulate a three-dimensional optical diffraction tomography experiment in which superresolution is achieved by illuminating the object with evanescent waves generated by a prism. We show that accounting for multiple scattering between the object and the prism interface is mandatory to obtain superresolved images. Because the Born approximation leads to poor results, we propose a nonlinear inversion method for retrieving the map of permittivity of the object from the scattered far field. We analyze the sensitivity to noise of our algorithm and point out the importance of using incident propagative waves together with evanescent waves to improve the robustness of the reconstruction without losing the superresolution.

Algorithms↗
PubMed2004

Coupled dipole method for scatterers with large permittivity.

In the coupled dipole method, a three-dimensional scattering object is discretized over a lattice into a set of polarizable units that are coupled self-consistently. Starting from the volume integral equation for the field, we show that performing the integration of the free-space field susceptibility tensor over the lattice cell dramatically improves the accuracy of the method when the permittivity of the object is large. This integration, done without any approximation, allows us to define a prescription for the polarizability used in the coupled dipole method. Our derivation is not restricted to any particular shape of the scatterer or to a cubic discretization lattice.

Journal Article↗
PubMed2002

Optical trapping and manipulation of nano-objects with an apertureless probe.

We propose a novel way to trap and manipulate nano-objects above a dielectric substrate using an apertureless near-field probe. A combination of evanescent illumination and light scattering at the probe apex is used to shape the optical field into a localized, three-dimensional optical trap. We use the coupled-dipole method and the Maxwell stress tensor to provide a self-consistent description of the optical force, including retardation and the influence of the substrate. We show that small objects can be selectively captured and manipulated under realistic conditions.

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