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Remo Nessler

Publications and source records attributed to Remo Nessler.

3 recordsLinked to original sources

Adaptation of dry nephelometer measurements to ambient conditions at the Jungfraujoch.

In a numerical study the influence of relative humidity (RH) on aerosol scattering coefficients sigma was investigated. Based on a core/coating aerosol model, RH enhancement factors for scattering, xi(RH) = sigma(RH)/sigma(RH = 0), were calculated for the wavelengths lambda = 450, 550, and 700 nm for a summer and a winter case. The investigation was adapted to the situation (e.g., chemical composition, particle size distributions, hygroscopic behavior) of the high-alpine site Jungfraujoch (JFJ, 3580 m asl), where long-term measurements of dry aerosol scattering coefficients are performed at these wavelengths. The presented results are therefore representative of the lower free troposphere above a continent. The RH enhancement factors at a specific RH strongly depend on the average particle size. For example, at RH = 85% they vary between approximately 1.2 and approximately 2.7 in summer and between approximately 1.4 and approximately 3.8 in winter. It is shown that there is a strong relationship between xi and the Angstrom exponent å (based on scattering only) of the dry aerosol, which is directly derived from the dry scattering measurements. This allows for parametrizing xi for a specific wavelength and season with å and RH. The parametrization is applicable for RH up to approximately 90%--for higher RH the underlying hygroscopic models become unreliable--and for å between approximately -0.25 and approximately 2.75, which covers the range observed at the JFJ. Also addressed is a systematic error in the dry scattering coefficients measured with a nephelometer previously discussed in the literature, which arises from nonidealities in the angular intensity distribution of the light inside the instrument. This effect also depends strongly on the particle size and can be described by a correction factor C that can be parametrized with å. The scattering coefficient corrected for measurement artifacts at ambient RH for specific wavelength and season therefore can be estimated from the uncorrected dry nephelometer scattering coefficient sigma(neph) as sigma(å, RH) = C(å) x xi(å, RH) x sigma(neph). As additional information only ambient RH data are needed. The 95% confidence bound of this total correction ranges from less than 5% for low RH and large å up to approximately 40% for high RH and small å.

Atmosphere↗

Microphysical aerosol parameters from multiwavelength lidar.

The hybrid regularization technique developed at the Institute of Mathematics of Potsdam University (IMP) is used to derive microphysical properties such as effective radius, surface-area concentration, and volume concentration, as well as the single-scattering albedo and a mean complex refractive index, from multiwavelength lidar measurements. We present the continuation of investigations of the IMP method. Theoretical studies of the degree of ill-posedness of the underlying model, simulation results with respect to the analysis of the retrieval error of microphysical particle properties from multiwavelength lidar data, and a comparison of results for different numbers of backscatter and extinction coefficients are presented. Our analysis shows that the backscatter operator has a smaller degree of ill-posedness than the operator for extinction. This fact underlines the importance of backscatter data. Moreover, the degree of ill-posedness increases with increasing particle absorption, i.e., depends on the imaginary part of the refractive index and does not depend significantly on the real part. Furthermore, an extensive simulation study was carried out for logarithmic-normal size distributions with different median radii, mode widths, and real and imaginary parts of refractive indices. The errors of the retrieved particle properties obtained from the inversion of three backscatter (355, 532, and 1064 nm) and two extinction (355 and 532 nm) coefficients were compared with the uncertainties for the case of six backscatter (400, 710, 800 nm, additionally) and the same two extinction coefficients. For known complex refractive index and up to 20% normally distributed noise, we found that the retrieval errors for effective radius, surface-area concentration, and volume concentration stay below approximately 15% in both cases. Simulations were also made with unknown complex refractive index. In that case the integrated parameters stay below approximately 30%, and the imaginary part of the refractive index stays below 35% for input noise up to 10% in both cases. In general, the quality of the retrieved aerosol parameters depends strongly on the imaginary part owing to the degree of ill-posedness. It is shown that under certain constraints a minimum data set of three backscatter coefficients and two extinction coefficients is sufficient for a successful inversion. The IMP algorithm was finally tested for a measurement case.

Journal Article↗

Development of a multiwavelength aerosol and water-vapor lidar at the Jungfraujoch Alpine Station (3580 m above sea level) in Switzerland.

The Jungfraujoch Research Station (46.55 degrees N, 7.98 degrees E, 3580 m above sea level) for decades has contributed in a significant manner to the systematic observation of the Earth's atmosphere both with in situ measurements and with trace gas column detection. We report on the development of a lidar system that improves the measurement potential of highly resolved atmospheric parameters in both time and space, with the goal of achieving long-term monitoring of atmospheric aerosol optical properties and water-vapor content. From the simultaneously detected elastic-backscatter signals at 355, 532, and 1064 nm, Raman signals from nitrogen at 387 and 607 nm, and water vapor at 408 nm, the aerosol extinction and backscatter coefficients at three wavelengths and a water-vapor mixing ratio are derived. Additional information about particle shape is obtained by depolarization measurements at 532 nm. Water-vapor measurements by use of both nitrogen and water-vapor Raman returns from the 355-nm laser beam are demonstrated with a vertical range resolution of 75 m and an integration time of 2 h. The comparison to the water-vapor profile derived from balloon measurements (Snow White technique) showed excellent agreement. The system design and the results obtained by its operation are reported.

Journal Article↗