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Radioactive wastes.

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Chemical Precipitation↗

General approach to dose reconstruction in the population exposed as a result of the release of radioactive wastes into the Techa River.

Massive releases of fission products from the plutonium production facility 'Mayak' resulted in the years 1949-1956 in the contamination of the river Techa and its flood lands. This led to the exposure of the population in many riverside villages due to external gamma-rays and due to the incorporation of radionuclides, primarily Sr-90. The exposure situation is described and the reconstruction of doses due to external and due to internal radioactivity is explained. The internal dosimetry is based on large scale measurements of Sr-90 beta-rays on the surface of teeth that were begun in 1960, and on whole-body measurements of Sr-90 that were begun in 1974. The details of the analyses are presented in Part 2 of the present report. Average doses due to the external and the internal exposure are given for the residents of the different villages along the river Techa. In the total population of about 28,000 persons that were assessed, the medium dose to the red bone marrow was about 0.25 Gy and the mean dose about 0.4 Gy. In about 5% of the individuals the dose to the red bone marrow was estimated to be in excess of 1 Gy.

Adolescent↗

Radioactive contamination in the marine environment adjacent to the outfall of the radioactive waste treatment plant at ATOMFLOT, northern Russia.

RTP "ATOMFLOT" is a civilian nuclear icebreaker base located on the Kola Bay of northwest Russia. The objectives of this study were to determine the distributions of man-made radionuclides in the marine environment adjacent to the base, to explain the form of the distributions in sediments and to derive information concerning the fate of radionuclides discharged from ATOMFLOT. Mean activity concentrations (d.w.) for surface sediment, of 63 Bq kg(-1 137Cs, 5.8 Bq kg(-1) 90Sr and 0.45 Bq kg(-1 239,240)Pu were measured. Filtered seawater activity levels were in the range of 3--6.9 Bq m(-3) 137Cs, 2.0-11.2 Bq m(-3) 90Sr, and 16-40 m Bq m(-3), 239,240Pu. Short-lived radionuclides were present at sediment depths in excess of 10cm indicating a high degree of sediment mixing. Correlations of radionuclide activity concentrations with grain-size appear to be absent; instead, the presence of relatively contaminated sediment appears to be related to the existence of radioactive particles.

Environmental Monitoring↗

Ramifications of risk measures in implementing quantitative performance assessment for the proposed radioactive waste repository at Yucca Mountain, Nevada, USA.

As part of its preparation to review a potential license application from the U.S. Department of Energy (DOE), the U.S. Nuclear Regulatory Commission (NRC) is examining the performance of the proposed Yucca Mountain nuclear waste repository. In this regard, we evaluated postclosure repository performance using Monte Carlo analyses with an NRC-developed system model that has 950 input parameters, of which 330 are sampled to represent system uncertainties. The quantitative compliance criterion for dose was established by NRC to protect inhabitants who might be exposed to any releases from the repository. The NRC criterion limits the peak-of-the-mean dose, which in our analysis is estimated by averaging the potential exposure at any instant in time for all Monte Carlo realizations, and then determining the maximum value of the mean curve within 10000 years, the compliance period. This procedure contrasts in important ways with a more common measure of risk based on the mean of the ensemble of peaks from each Monte Carlo realization. The NRC chose the former (peak-of-the-mean) because it more correctly represents the risk to an exposed individual. Procedures for calculating risk in the expected case of slow repository degradation differ from those for low-probability cases of disruption by external forces such as volcanism. We also explored the possibility of risk dilution (i.e., lower calculated risk) that could result from arbitrarily defining wide probability distributions for certain parameters. Finally, our sensitivity analyses to identify influential parameters used two approaches: (1). the ensemble of doses from each Monte Carlo realization at the time of the peak risk (i.e., peak-of-the-mean) and (2). the ensemble of peak doses calculated from each realization within 10000 years. The latter measure appears to have more discriminatory power than the former for many parameters (based on the greater magnitude of the sensitivity coefficient), but can yield different rankings, especially for parameters that influence the timing of releases.

Journal Article↗

Correction factors in the EPR dose reconstruction for residents of the Middle and Lower Techa riverside.

During 1949-1956, the first Soviet nuclear weapons plant, Mayak, released about 7.6 x 10(7) m(-3) of liquid radioactive waste with a total activity of 10(17) Bq into the Techa River (Southern Urals, Russia). 90Sr contributed 11.6% to the total waste radioactivity. As a result of these radioactive discharges, about 28,000 local residents were exposed to ionizing radiation, and some of them received relatively high doses. Internal exposure of the population residing at the Middle and Lower Techa riverside was mostly from 90Sr deposited in bone and tooth tissues. In order to reconstruct radiation doses to this population group, a study of 35 teeth extracted from local residents was carried out using electron paramagnetic resonance measurements. A total of 73 samples from these 35 teeth (tooth enamel, 33; crown dentin, 20; and root dentin, 20) were prepared and measured with electron paramagnetic resonance. The study revealed high doses (up to 15 Gy) absorbed in tooth enamel of the individuals born during 1945-1949, which was attributed to very high local 90Sr concentration in tooth enamel of this particular age group in the population. The analysis presented here takes into account (a) the time courses both of the release/intake of 90Sr and of the tooth formation, and (b) expected variations in measured absorbed doses due to differing geometric sizes of tooth structures. This methodology enables a more consistent picture to be developed of the 90Sr intake by the Middle and Lower Techa riverside population, based on electron paramagnetic resonance tooth dosimetry.

Age Factors↗

[Physico-chemical and microbiological characteristics of groundwater from observation boreholes of a deep radioactive liquid waste repository].

A radioactive liquid waste repository was found to be a habitat of the rich microbial community with a high catabolic potential. Groundwater from a depth of 162-189 m contained aerobic saprotrophic and anaerobic fermentative, sulfate-reducing, and denitrifying bacteria. Nitrate-reducing bacteria residing in this groundwater were isolated in pure cultures. Based on the results of their physiological studies, 16S rRNA sequencing, and phylogenetic analysis, the microorganisms isolated were ascribed to one phylogenetic branch, the gamma-subclass of gram-negative bacteria. Among six isolates, four belonged to the genus Acinetobacter, whereas two others belonged to the genera Comamonas and Aeromonas. The data obtained indicate that the microflora of the repository can exert a certain effect on the chemical composition of the formation fluids and bearing rocks, as well as on the migration of radionuclides.

Bacteria↗

Potential for radioactive patient excreta in hospital trash and medical waste.

Radioactive excreta from nuclear medicine patients can enter solid waste as common trash and medical biohazardous waste. Many landfills and transfer stations now survey these waste streams with scintillation detectors which may result in rejection of a hospital's waste. Our survey indicated that on the average either or both of Boston University Medical Center Hospital's waste streams can contain detectable radioactive excreta on a weekly basis. To avoid potential problems, radiation detectors were installed in areas where housekeepers carting trash and medical waste must pass through to ensure no radioactivity leaves the institution.

Housekeeping, Hospital↗

Autoclave inactivation of infectious radioactive laboratory waste contained within a charcoal filtration system.

A model system was developed previously for disposal of solid laboratory waste that is both radioactive and heat sensitive, e.g., HIV. A double polypropylene bag with charcoal vent filter and absorbent was designed to meet requirements for both steam sterilization and disposal as solid radioactive waste. Earlier work demonstrated the effective containment of radioactive gases by the filter and inactivation of organisms as heat sensitive as HIV. We sought to broaden the application of this model to ensure inactivation of microorganisms that are more heat resistant than HIV. The efficacy of steam sterilization using water or solutions of iodophor, hypochlorite, or hydrogen peroxide was studied under constant temperature and time conditions. The systems were monitored with internal probes, physical, chemical, and biological indicators. Biological indicators documented inactivation when bags containing hydrogen peroxide (3%) were autoclaved for 60 min at 121 degrees C. Synergistic activity between hydrogen peroxide and autoclave conditions significantly reduced processing time.

Charcoal↗

Engineering Deinococcus radiodurans for metal remediation in radioactive mixed waste environments.

We have developed a radiation resistant bacterium for the treatment of mixed radioactive wastes containing ionic mercury. The high cost of remediating radioactive waste sites from nuclear weapons production has stimulated the development of bioremediation strategies using Deinococcus radiodurans, the most radiation resistant organism known. As a frequent constituent of these sites is the highly toxic ionic mercury (Hg) (II), we have generated several D. radiodurans strains expressing the cloned Hg (II) resistance gene (merA) from Escherichia coli strain BL308. We designed four different expression vectors for this purpose, and compared the relative advantages of each. The strains were shown to grow in the presence of both radiation and ionic mercury at concentrations well above those found in radioactive waste sites, and to effectively reduce Hg (II) to the less toxic volatile elemental mercury. We also demonstrated that different gene clusters could be used to engineer D. radiodurans for treatment of mixed radioactive wastes by developing a strain to detoxify both mercury and toluene. These expression systems could provide models to guide future D. radiodurans engineering efforts aimed at integrating several remediation functions into a single host.

Bacterial Proteins↗

[Introduction of manual for the management radioactive medical waste].

Societies concerned with radioactive rays and nuclear medicine have recently highlighted the necessity of managing radioactive medical waste resulting from nuclear medicine examinations. We introduce a manual that we have created and explain its use in decision-making and management practices aimed at the reduction of radioactive medical waste at hospitals that have not yet solved this problem. We hope that our manual will help in reducing this medical waste.

Japan↗

Treatment of radioactive liquid waste by sorption on natural zeolite in Turkey.

Liquid radioactive waste has been generated from the use of radioactive materials in industrial applications, research and medicine in Turkey. Natural zeolites (clinoptilolite) have been studied for the removal of several key radionuclides ((137)Cs, (60)Co, (90)Sr and (110m)Ag) from liquid radioactive waste. The aim of the present study is to investigate effectiveness of zeolite treatment on decontamination factor (DF) in a combined process (chemical precipitation and adsorption) at the laboratory tests and scale up to the waste treatment plant. In this study, sorption and precipitation techniques were adapted to decontamination of liquid low level waste (LLW). Effective decontamination was achieved when sorbents are used during the chemical precipitation. Natural zeolite samples were taken from different zeolite formations in Turkey. Comparison of the ion-exchange properties of zeolite minerals from different formations shows that Gordes clinoptilolite was the most suitable natural sorbent for radionuclides under dynamic treatment conditions and as an additive for chemical precipitation process. Clinoptilolite were shown to have a high selectivity for (137)Cs and (110m)Ag as sorbent. In the absence of potassium ions, native clinoptilolite removed (60)Co and (90)Sr very effectively from the liquid waste. In the end of this liquid waste treatment, decontamination factor was provided as 430 by using 0.5 mm clinoptilolite at 30 degrees C.

Adsorption↗