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Stability of a mass accreting shell expanding in a plasma.

A linearized analysis is presented of the stability of a shell which accretes mass as it expands in a plasma under the push of the electromagnetic radiation trapped inside it. The interaction with the radiation is described in terms of a ponderomotive force and the shell dynamics is treated within the snowplow approximation. The mass accretion and the radiation expansion are shown to affect the stability of planar, cylindrical, and spherical shells differently.

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K-shell spectroscopy of an independently diagnosed uniaxially expanding laser-produced aluminum plasma.

We present detailed spectroscopic analysis of the primary K-shell emission lines from a uniaxially expanding laser-produced hydrogenic and heliumlike aluminum plasma. The spectroscopic measurements are found to be consistent with time-dependent hydrodynamic properties of the plasma, measured using Thomson scattering and shadowgraphy. The K-shell population kinetics code FLY with the measured hydrodynamic parameters is used to generate spectra that are compared to the experimental spectra. Excellent agreement is found between the measured and calculated spectra for a variety of experimental target widths employed to produce plasmas with different optical depths. The peak emission from the hydrogenic Lyman series is determined to be from a temporal and spatial region where the hydrodynamic parameters are essentially constant. This allows a single steady-state solution of FLY to be used to deduce the electron temperature and density, from the measured line ratios and linewidths, for comparison with the Thomson and shadowgraphy data. These measurements are found to agree well with time-dependent calculations, and provide further validation for the FLY calculations of the ionization and excitation balance for a K-shell aluminum plasma. We also discuss the possible application of this data as a benchmark for hydrodynamic simulations and ionization/excitation balance calculations.

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Hot-electron influence on L-shell spectra of multicharged Kr ions generated in clusters irradiated by femtosecond laser pulses.

Strong L-shell x-ray emission has been obtained from Kr clusters formed in gas jets and irradiated by 60-500-fs laser pulses. Spectral lines from the F-, Ne- Na-, and Mg-like charge states of Kr have been identified from highly resolved x-ray spectra. Spectral line intensities are used in conjunction with a detailed time-dependent collisional-radiative model to diagnose the electron distribution functions of plasmas formed in various gas jet nozzles with various laser pulse durations. It is shown that L-shell spectra formed by relatively long nanosecond-laser pulses can be well described by a steady-state model without hot electrons when opacity effects are included. In contrast, adequate modeling of L-shell spectra from highly transient and inhomogeneous femtosecond-laser plasmas requires including the influence of hot electrons. It is shown that femtosecond-laser interaction with gas jets from conical nozzles produces plasmas with higher ionization balances than plasmas formed by gas jets from Laval nozzles, in agreement with previous work for femtosecond laser interaction with Ar clusters.

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Advanced spectroscopic analysis of 0.8-1.0-MA Mo x pinches and the influence of plasma electron beams on L-shell spectra of Mo ions.

This paper presents a detailed investigation of the temporal, spatial, and spectroscopic properties of L-shell radiation from 0.8 to 1.0 MA Mo x pinches. Time-resolved measurements of x-ray radiation and both time-gated and time-integrated spectra and pinhole images are presented and analyzed. High-current x pinches are found to have complex spatial and temporal structures. A collisional-radiative kinetic model has been developed and used to interpret L-shell Mo spectra. The model includes the ground state of every ionization stage of Mo and detailed structure for the O-, F-, Ne-, Na-, and Mg-like ionization stages. Hot electron beams generated by current-carrying electrons in the x pinch are modeled by a non-Maxwellian electron distribution function and have significant influence on L-shell spectra. The results of 20 Mo x-pinch shots with wire diameters from 24 to 62 microm have been modeled. Overall, the modeled spectra fit the experimental spectra well and indicate for time-integrated spectra electron densities between 2 x 10(21) and 2 x 10(22) cm(-3), electron temperatures between 700 and 850 eV, and hot electron fractions between 3% and 7%. Time-gated spectra exhibit wide variations in temperature and density of plasma hot spots during the same discharge.

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Unstable periodic solutions embedded in a shell model turbulence.

An approach to intermittency of a shell model turbulence is proposed from the viewpoint of dynamical systems. We detected unstable solutions of the Gledzer-Ohkitani-Yamada shell model and studied their relation to turbulence statistics. One of the solutions has an unstable periodic orbit (UPO), which shows an intermittency where the scaling exponents of the structure function have a nonlinear dependence on its order, quite similar to that of turbulence solution at the same parameter values. The attractor in the phase space is found to be well approximated by a continuous set of solutions generated from the UPO through a one-parameter phase transformation, which implies that the intermittency of the shell model turbulence is described by this UPO.

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Virus shapes and buckling transitions in spherical shells.

We show that the icosahedral packings of protein capsomeres proposed by Caspar and Klug for spherical viruses become unstable to faceting for sufficiently large virus size, in analogy with the buckling instability of disclinations in two-dimensional crystals. Our model, based on the nonlinear physics of thin elastic shells, produces excellent one-parameter fits in real space to the full three-dimensional shape of large spherical viruses. The faceted shape depends only on the dimensionless Foppl-von Kármán number gamma=YR(2)/kappa, where Y is the two-dimensional Young's modulus of the protein shell, kappa is its bending rigidity, and R is the mean virus radius. The shape can be parametrized more quantitatively in terms of a spherical harmonic expansion. We also investigate elastic shell theory for extremely large gamma, 10(3)<gamma<10(8), and find results applicable to icosahedral shapes of large vesicles studied with freeze fracture and electron microscopy.

Crystallography, X-Ray↗

Breakup of shells under explosion and impact.

A theoretical and experimental study of the fragmentation of closed thin shells made of a disordered brittle material is presented. Experiments were performed on eggshells under two different loading conditions: fragmentation due to an impact with a hard wall and explosion by a combustion mixture giving rise to power law fragment size distributions. For the theoretical investigations a three-dimensional discrete element model of shells is constructed. Molecular dynamics simulations of the two loading cases resulted in power law fragment mass distributions in satisfactory agreement with experiments. Based on large scale simulations we give evidence that power law distributions arise due to an underlying phase transition which proved to be abrupt and continuous for explosion and impact, respectively. Our results demonstrate that the fragmentation of closed shells defines a universality class, different from that of two- and three-dimensional bulk systems.

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Multiplicity of nonlinear thermal convection in a spherical shell.

Linear and weakly nonlinear thermal convection in a moderately thin spherical shell in the presence of a spherically symmetric gravity subject to a spherically symmetric boundary condition is systematically investigated through fully three-dimensional numerical simulations. The convection problem is self-adjoint and the linear convective stability is characterized by l, the degree of a spherical harmonics Yml (theta,phi). While the radial structure of the linear convection is determined by the stability analysis, there exists a (2l + 1)-fold degeneracy in the horizontal structure of the spherical convection. When l = O(10) , i.e., in a moderately thin spherical shell, the removal or partial removal of the degeneracy represents a mathematically difficult, physically not well-understood problem. By starting with carefully chosen initial conditions, we are able to obtain a variety of nonlinear convective flows at exactly the same parameters near the onset of convection, including steady axisymmetric convection, steady azimuthally periodic convection, steady azimuthally nonperiodic convection, equatorially asymmetric convection, and steady convection in the form of a single giant spiral roll covering the whole spherical shell which is stable and robust for a wide range of the Prandtl number.

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Elasticity theory and shape transitions of viral shells.

Recently, continuum elasticity theory has been applied to explain the shape transition of icosahedral viral capsids--single-protein-thick crystalline shells--from spherical to "buckled" or faceted as their radius increases through a critical value determined by the competition between stretching and bending energies of a closed two-dimensional (2D) elastic network. In the present work we generalize this approach to capsids with nonicosahedral symmetries, e.g., spherocylindrical and conical shells. One key additional physical ingredient is the role played by nonzero spontaneous curvature. Another is associated with the special way in which the energy of the 12 topologically required fivefold sites depends on the "background" local curvature of the shell in which they are embedded. Systematic evaluation of these contributions leads to a shape "phase" diagram in which transitions are observed from icosahedral to spherocylindrical capsids as a function of the ratio of stretching to bending energies and of the spontaneous curvature of the 2D protein network. We find that the transition from icosahedral to spherocylindrical symmetry is continuous or weakly first order near the onset of buckling, leading to extensive shape degeneracy. These results are discussed in the context of experimentally observed variations in the shapes of a variety of viral capsids.

Capsid↗

Progress toward ignition with noncryogenic double-shell capsules

Inertial confinement fusion implosions using capsules with two concentric shells separated by a low density region (double shells) are reported which closely follow one dimensional (1D) radiatively driven hydrodynamics simulations. Capsule designs which mitigate Au M-band radiation asymmetries appear to correspond more closely to 1D simulations than targets lacking mitigation of hohlraum drive M-band nonuniformities. One capsule design achieves over 50% of the unperturbed 1D calculated yield at a convergence ratio of 25.5, comparable to that of a double-shell design for an ignition capsule at the National Ignition Facility.

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Experimental evidence of threshold effects in the energy loss of protons in carbon and aluminum due to inner shell ionization

We explore the contributions of inner shell ionization to the energy loss of 7 to 270 keV protons in C and Al foils under experimental conditions such that the product of the observation angle and the projectile energy is kept constant. By normalizing these energy loss measurements to the energy loss in the forward direction we observe a pronounced rising behavior with increasing energy. This effect appears in the same range of energies where the respective K- and L-shell ionization cross sections of these elements show a similar threshold behavior. Based also on various theoretical considerations we interpret these results as clear evidence of the inner shell ionization contribution to the energy loss.

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Spin-orbit matrix elements in the atomic f shell from automorphisms of SO(8)

A scrutiny of the matrix elements within the f shell of the spin-other-orbit interaction H(soo) has revealed many unexpected proportionalities that go beyond an application of the Wigner-Eckart theorem to Racah's groups G2 and SO(7). An explanation is sought by using the automorphisms of SO(8) by means of which the states of the atomic f shell are generated by two alternative SO(7) bases of the type (1 / 21 / 21 / 2)(4), each augmented by two parity labels. Transformations between the bases can be made by reversing the relative phases of the two angular-momentum states 3 and 0 that comprise any one of the four SO(7) spinors. The method is exemplified by the single-electron spin-orbit interaction H(so), for which a component can be found that is invariant under the phase reversal. The extension from H(so) to H(soo) is described for the component z(6) of H(soo), and several examples drawn from the comparatively inaccessible configurations near the middle of the f shell are presented.

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Evolution of shell nonuniformities near peak compression of a spherical implosion.

The evolution of shell modulations near peak compression of direct-drive spherical-target implosions has been measured using the 60-beam, 30-kJ UV OMEGA laser system. The spatial size and amplitude of shell-areal-density modulations decrease during the target compression, then increase during its decompression as expected. The shell uniformity at peak compression has been increased by reducing single-beam, laser-drive nonuniformity.

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Shell filling in closed single-wall carbon nanotube quantum dots.

We observe twofold shell filling in the spectra of closed one-dimensional quantum dots formed in single-wall carbon nanotubes. Its signatures include a bimodal distribution of addition energies, correlations in the excitation spectra for different electron number, and alternation of the spins of the added electrons. This provides a contrast with quantum dots in higher dimensions, where such spin pairing is absent. We also see indications of an additional fourfold periodicity indicative of K-K' subband shells. Our results suggest that the absence of shell filling in most isolated nanotube dots results from disorder or nonuniformity.

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Inverse cascade regime in shell models of two-dimensional turbulence.

We consider shell models that display an inverse energy cascade similar to two-dimensional turbulence (together with a direct cascade of an enstrophylike invariant). Previous attempts to construct such models ended negatively, stating that shell models give rise to a "quasiequilibrium" situation with equipartition of the energy among the shells. We show analytically that the quasiequilibrium state predicts its own disappearance upon changing the model parameters in favor of the establishment of an inverse cascade regime with Kolmogorov scaling. The latter regime is found where predicted, offering a useful model to study inverse cascades.

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Shell mix in the compressed core of spherical implosions.

The Rayleigh-Taylor instability in its highly nonlinear, turbulent stage causes atomic-scale mixing of the shell material with the fuel in the compressed core of inertial-confinement fusion targets. The density of shell material mixed into the outer core of direct-drive plastic-shell spherical-target implosions on the 60-beam, OMEGA laser system is estimated to be 3.4(+/-1.2) g/cm(3) from time-resolved x-ray spectroscopy, charged-particle spectroscopy, and core x-ray images. The estimated fuel density, 3.6(+/-1) g/cm(3), accounts for only approximately 50% of the neutron-burn-averaged electron density, n(e)=2.2(+/-0.4)x10(24) cm(-3).

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Lowest excitations in 56Ti and the predicted N=34 shell closure.

Recent experimental characterization of the subshell closure at N=32 in the Ca, Ti, and Cr isotones has stimulated shell-model calculations that indicated the possibility that the N=34 isotones of these same elements could exhibit characteristics of a shell closure, namely, a high energy for the first excited 2(+) level. To that end, we have studied the decay of 56Sc produced in fragmentation reactions and identified new gamma rays in the daughter N=34 isotone 56Ti. The first 2(+) level is found at an energy of 1127 keV, well below the expected position that would indicate the presence of an N=34 shell closure in 56Ti.

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Coulomb-interaction-induced incomplete shell filling in the hole system of InAs quantum dots.

We have studied the hole charging spectra of self-assembled InAs quantum dots in perpendicular magnetic fields by capacitance-voltage spectroscopy. From the magnetic-field dependence of the individual peaks we conclude that the s-like ground state is completely filled with two holes but that the fourfold degenerate p shell is only half filled with two holes before the filling of the d shell starts. The resulting six-hole ground state is highly polarized. This incomplete shell filling can be explained by the large influence of the Coulomb interaction in this system.

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